Adamiak D A, Rypniewski W R, Milecki J, Adamiak R W
Institute of Bioorganic Chemistry, Polish Academy of Sciences, Noskowskiego 12-14, 61-704 Poznañ, Poland.
Nucleic Acids Res. 2001 Oct 15;29(20):4144-53. doi: 10.1093/nar/29.20.4144.
The crystal and molecular structure of 2'-O-Me(CGCGCG)(2) has been determined at 1.19 A resolution, at 100 K, using synchrotron radiation. The structure in space group P3(2)12 is a half-turn right-handed helix that includes two 2-methyl-2,4-pentanediol (MPD) molecules bound in the minor groove. The structure deviates from A-form RNA. The duplex is overwound with an average value of 9.7 bp per turn, characterised as having a C3'-endo sugar pucker, very low base pair rise and high helical twist and inclination angles. The structure includes 65 ordered water molecules. Only a single row of water molecules is observed in the minor groove due to the presence of hydrophobic 2'-O-methyl groups. As many as five magnesium ions are located in the structure. Two are in the major groove and interact with O(6) and N(7) of guanosine and N(4) of cytidine residues through their hydration spheres. This work provides the first example of molecular interactions of nucleic acids with MPD, which was used as a precipitant, cryo-solvent and resolution enhancing agent. The two MPD molecules intrude into the hydration network in the minor groove, each forming hydrogen bonds between their secondary hydroxyl group and exo-amino functions of guanosine residues. Comparison of the 2'-O-Me(CGCGCG)(2) structure in the P3(2)12 and P6(1)22 crystals delineates stability of the water network within the minor groove to dehydration by MPD and is of interest for evaluating factors governing small molecule binding to RNA. Intrusion of MPD into the minor groove of 2'-O-Me(CGCGCG)(2) is discussed with respect to RNA dehydration, a prerequisite of Z-RNA formation.
利用同步辐射,在100 K下以1.19 Å的分辨率测定了2'-O-Me(CGCGCG)(2)的晶体和分子结构。空间群为P3(2)12的结构是一个半圈右手螺旋,其中包括两个结合在小沟中的2-甲基-2,4-戊二醇(MPD)分子。该结构不同于A-型RNA。双链过度缠绕,平均每圈9.7个碱基对,其特征为具有C3'-内型糖构象、非常低的碱基对上升以及高螺旋扭转和倾斜角。该结构包含65个有序水分子。由于存在疏水性的2'-O-甲基基团,在小沟中仅观察到单排水分子。结构中定位了多达五个镁离子。两个在大沟中,通过它们的水合球与鸟苷的O(6)和N(7)以及胞苷残基的N(4)相互作用。这项工作提供了核酸与MPD分子相互作用的首个实例,MPD用作沉淀剂、低温溶剂和分辨率增强剂。两个MPD分子侵入小沟中的水合网络,各自在其次级羟基与鸟苷残基的外氨基官能团之间形成氢键。P3(2)12和P6(1)22晶体中2'-O-Me(CGCGCG)(2)结构的比较描绘了小沟内水网络对MPD脱水的稳定性,对于评估控制小分子与RNA结合的因素具有重要意义。关于RNA脱水(Z-RNA形成的一个先决条件),讨论了MPD侵入2'-O-Me(CGCGCG)(2)小沟的情况。