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土壤中铯-137的垂直分布

Vertical profile of 137Cs in soil.

作者信息

Krstić D, Nikezić D, Stevanović N, Jelić M

机构信息

University of Kragujevac, Faculty of Science, R.Domanovica 12 Kragujevac 34000, Serbia and Montenegro.

出版信息

Appl Radiat Isot. 2004 Dec;61(6):1487-92. doi: 10.1016/j.apradiso.2004.03.118.

Abstract

In this paper, a vertical distribution of 137Cs in undisturbed soil was investigated experimentally and theoretically. Soil samples were taken from the surroundings of the city of Kragujevac in central Serbia during spring-summer of 2001. The sampling locations were chosen in such a way that the influence of soil characteristics on depth distribution of 137Cs in soil could be investigated. Activity of 137Cs in soil samples was measured using a HpGe detector and multi-channel analyzer. Based on vertical distribution of 137Cs in soil which was measured for each of 10 locations, the diffusion coefficient of 137Cs in soil was determined. In the next half-century, 137Cs will remain as the source of the exposure. Fifteen years after the Chernobyl accident, and more than 30 years after nuclear probes, the largest activity of 137Cs is still within 10 cm of the upper layer of the soil. This result confirms that the penetration of 137Cs in soil is a very slow process. Experimental results were compared with two different Green functions and no major differences were found between them. While both functions fit experimental data well in the upper layer of soil, the fitting is not so good in deeper layers. Although the curves obtained by these two functions are very close to each other, there are some differences in the values of parameters acquired by them.

摘要

本文通过实验和理论研究了未扰动土壤中¹³⁷Cs的垂直分布。2001年春夏期间,从塞尔维亚中部克拉古耶瓦茨市周边采集土壤样本。采样地点的选择方式使得能够研究土壤特性对土壤中¹³⁷Cs深度分布的影响。使用高纯锗探测器和多道分析仪测量土壤样本中¹³⁷Cs的活度。根据在10个地点分别测量的土壤中¹³⁷Cs的垂直分布,确定了¹³⁷Cs在土壤中的扩散系数。在接下来的半个世纪里,¹³⁷Cs仍将是辐射源。切尔诺贝利事故发生15年后,以及核探测30多年后,¹³⁷Cs的最大活度仍在土壤上层10厘米范围内。这一结果证实¹³⁷Cs在土壤中的渗透是一个非常缓慢的过程。将实验结果与两种不同的格林函数进行了比较,未发现它们之间有重大差异。虽然这两种函数在上层土壤中都能很好地拟合实验数据,但在较深层的拟合效果不太好。尽管由这两种函数得到的曲线彼此非常接近,但它们获得的参数值存在一些差异。

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