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贝尔格莱德地区地面空气中7Be与210Pb的浓度比。

7Be to 210Pb concentration ratio in ground level air in Belgrade area.

作者信息

Todorovic D, Popovic D, Djuric G, Radenkovic M

机构信息

Environmental and Radiation Protection Laboratory, Institute of Nuclear Sciences Vinca, P.O. Box 522, 11001 Belgrade, Serbia and Montenegro.

出版信息

J Environ Radioact. 2005;79(3):297-307. doi: 10.1016/j.jenvrad.2004.08.003.

Abstract

7Be to 210Pb concentration ratios in ground level air on two monitoring stations (MS1 and MS2) in Belgrade area were determined from 1996 to 2001. The average monthly concentrations of 7Be in ground level air were in the range of 0.6-18.3 mBq/m3 and exhibited one or two summer/early fall maxims and one minimum in winter. The maximum concentrations for 210Pb were generally observed in the fall, with the average concentrations in the range of 1.09 x 10(-4) to 30.9 x 10(-4) Bq/m3. The 7Be/210Pb ratios were in the range of 1.7-12.7 (MS1) and 1.8-11.3 (MS2), with summer maxims and late fall/winter minimums. The mean Radionuclides Loading Indices values approach zero except for 1996/1997 (MS1) and 2001 (MS2) due to higher concentrations of 7Be and 210Pb. The mean monthly concentrations of both radionuclides exhibited lognormal distributions. There is significant correlation between the 7Be/210Pb activities ratio and the air stability classes A + B + C for both monitoring stations (correlation coefficients 0.61-0.65), and no correlation with D class and E + F classes. Correlation was found between the activity of 7Be and air stability classes A + B + C (0.46-0.68), and E + F (0.38 for MS1), while for 210Pb, a moderate correlation (0.38-0.40) was found with the E + F air stability classes.

摘要

1996年至2001年期间,测定了贝尔格莱德地区两个监测站(MS1和MS2)地面空气中7Be与210Pb的浓度比。地面空气中7Be的月平均浓度在0.6 - 18.3 mBq/m³范围内,呈现出一个或两个夏季/初秋最大值以及一个冬季最小值。210Pb的最大浓度通常出现在秋季,平均浓度在1.09×10⁻⁴至30.9×10⁻⁴ Bq/m³范围内。7Be/210Pb比值在1.7 - 12.7(MS1)和1.8 - 11.3(MS2)范围内,呈现夏季最大值以及深秋/冬季最小值。除了1996/1997年(MS1)和2001年(MS2)由于7Be和210Pb浓度较高外,平均放射性核素负荷指数值接近零。两种放射性核素的月平均浓度均呈现对数正态分布。两个监测站的7Be/210Pb活度比与空气稳定等级A + B + C之间存在显著相关性(相关系数为0.61 - 0.65),与D级以及E + F级无相关性。发现7Be活度与空气稳定等级A + B + C(0.46 - 0.68)以及E + F(MS1为0.38)之间存在相关性,而对于210Pb,与E + F空气稳定等级存在中等相关性(0.38 - 0.40)。

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