Walls Jamie D, Heller Eric J
Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138, USA.
Nano Lett. 2007 Nov;7(11):3377-82. doi: 10.1021/nl071711z. Epub 2007 Oct 4.
Lack of inversion symmetry at a metallic surface can lead to an observable spin-orbit interaction. For certain metal surfaces, such as the Au(111) surface, the experimentally observed spin-orbit coupling results in spin rotation lengths on the order of tens of nanometers, which is the typical length scale associated with quantum corral structures formed on metal surfaces. In this work, multiple scattering theory is used to calculate the local density of states (LDOS) of quantum corral structures composed of nonmagnetic adatoms in the presence of spin-orbit coupling. Contrary to previous theoretical predictions, spin-orbit coupling induced modulations are observed in the theoretical LDOS, which should be observable using scanning tunneling microscopy.
金属表面缺乏反演对称性会导致可观测的自旋 - 轨道相互作用。对于某些金属表面,如金(111)表面,实验观测到的自旋 - 轨道耦合会导致自旋旋转长度达到几十纳米量级,这是与在金属表面形成的量子围栏结构相关的典型长度尺度。在这项工作中,多重散射理论被用于计算在存在自旋 - 轨道耦合的情况下由非磁性吸附原子组成的量子围栏结构的局域态密度(LDOS)。与先前的理论预测相反,在理论LDOS中观测到了自旋 - 轨道耦合诱导的调制,这应该可以通过扫描隧道显微镜观测到。