Krellner C, Förster T, Jeevan H, Geibel C, Sichelschmidt J
Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany.
Phys Rev Lett. 2008 Feb 15;100(6):066401. doi: 10.1103/PhysRevLett.100.066401. Epub 2008 Feb 11.
Electron spin resonance (ESR) measurements of the ferromagnetic (FM) Kondo lattice system CeRuPO show a well defined ESR signal which is related to the Ce3+ magnetism. In contrast, no ESR could be observed in the antiferromagnetic (AFM) homologue CeOsPO. Additionally, we detect an ESR signal in ferromagnetic YbRh while it was absent in a number of Ce or Yb intermetallic compounds with dominant AFM exchange. Thus, the observation of an ESR signal in a Kondo lattice is neither specific to Yb nor to the proximity to a quantum critical point, but seems to be connected to the presence of FM fluctuations. These conclusions not only provide a basic concept to understand the ESR in Kondo lattice systems even well below the Kondo temperature (as observed in YbRh2Si2) but point out ESR as a prime method to investigate directly the spin dynamics of the Kondo ion.
对铁磁(FM)近藤晶格体系CeRuPO进行的电子自旋共振(ESR)测量显示出一个明确的ESR信号,该信号与Ce3+磁性有关。相比之下,在反铁磁(AFM)同系物CeOsPO中未观察到ESR信号。此外,我们在铁磁YbRh中检测到一个ESR信号,而在许多具有主导AFM交换的Ce或Yb金属间化合物中该信号不存在。因此,在近藤晶格中观察到ESR信号既不是Yb所特有的,也不是与量子临界点的接近程度所特有的,而是似乎与FM涨落的存在有关。这些结论不仅为理解近藤晶格体系中甚至远低于近藤温度(如在YbRh2Si2中观察到的)的ESR提供了一个基本概念,而且指出ESR是直接研究近藤离子自旋动力学的主要方法。