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哈伯德纳米团簇中的自旋-电荷分离与电子配对不稳定性

Spin-charge separation and electron pairing instabilities in Hubbard nanoclusters.

作者信息

Kocharian A N, Fernando G W, Palandage K, Davenport J W

机构信息

Department of Physics, California State University, Los Angeles, CA 90032, USA.

出版信息

Ultramicroscopy. 2009 Jul;109(8):1066-73. doi: 10.1016/j.ultramic.2009.03.032. Epub 2009 Mar 21.

Abstract

Electron charge and spin pairing instabilities in various cluster geometries for attractive and repulsive electrons are studied exactly under variation of interaction strength, electron doping and temperature. The exact diagonalization, level crossing degeneracies, spin-charge separation and separate condensation of paired electron charge and opposite spins yield intriguing insights into the origin of magnetism, ferroelectricity and superconductivity seen in inhomogeneous bulk nanomaterials and various phenomena in cold fermionic atoms in optical lattices. Phase diagrams resemble a number of inhomogeneous, coherent and incoherent nanoscale phases found recently in high-T(c) cuprates, manganites and multiferroic nanomaterials probed by scanning tunneling microscopy. Separate condensation of electron charge and spin degrees at various crossover temperatures offers a new route for superconductivity, different from the BCS scenario. The calculated phase diagrams resemble a number of inhomogeneous paired phases, superconductivity, ferromagnetism and ferroelectricity found in Nb and Co nanoparticles. The phase separation and electron pairing, monitored by electron doping and magnetic field surprisingly resemble incoherent electron pairing in the family of doped high-T(c) cuprates, ruthenocuprates, iron pnictides and spontaneous ferroelectricity in multiferroic materials.

摘要

在相互作用强度、电子掺杂和温度变化的情况下,精确研究了吸引电子和排斥电子在各种团簇几何结构中的电子电荷和自旋配对不稳定性。精确对角化、能级交叉简并、自旋 - 电荷分离以及成对电子电荷和相反自旋的单独凝聚,为非均匀体纳米材料中观察到的磁性、铁电性和超导性的起源以及光学晶格中冷费米子原子的各种现象提供了有趣的见解。相图类似于最近在高温超导体铜酸盐、锰酸盐和多铁性纳米材料中通过扫描隧道显微镜探测到的许多非均匀、相干和非相干纳米级相。在各种交叉温度下电子电荷和自旋自由度的单独凝聚为超导性提供了一条不同于BCS理论的新途径。计算得到的相图类似于在铌和钴纳米颗粒中发现的许多非均匀配对相、超导性、铁磁性和铁电性。通过电子掺杂和磁场监测的相分离和电子配对,令人惊讶地类似于掺杂高温超导体铜酸盐、钌铜酸盐、铁基磷化物家族中的非相干电子配对以及多铁性材料中的自发铁电性。

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