Bobroff J, Laflorencie N, Alexander L K, Mahajan A V, Koteswararao B, Mendels P
Laboratoire de Physique des Solides, Université Paris-Sud, UMR-8502 CNRS, 91405 Orsay, France.
Phys Rev Lett. 2009 Jul 24;103(4):047201. doi: 10.1103/PhysRevLett.103.047201. Epub 2009 Jul 21.
We have studied the effect of nonmagnetic Zn impurities in the coupled spin ladder Bi(Cu_{1-x}Zn_{x}){2}PO{6} using ;{31}P NMR, muon spin resonance (microSR), and quantum Monte Carlo simulations. Our results show that the impurities induce in their vicinity antiferromagnetic polarizations, extending over a few unit cells. At low temperature, these extended moments freeze in a process which is found universal among various other spin-gapped compounds: isolated ladders, Haldane, or spin-Peierls chains. This allows us to propose a simple common framework to explain the generic low-temperature impurity-induced freezings observed in low-dimensional spin-gapped materials.
我们利用³¹P核磁共振、μ子自旋共振(μSR)以及量子蒙特卡罗模拟,研究了耦合自旋梯状化合物Bi(Cu₁₋ₓZnₓ)₂PO₆中无磁性Zn杂质的影响。我们的结果表明,杂质在其附近诱导出反铁磁极化,这种极化延伸几个晶胞。在低温下,这些扩展的磁矩会冻结,这一过程在其他各种自旋能隙化合物中普遍存在:孤立的自旋梯、霍尔丹链或自旋-派尔斯链。这使我们能够提出一个简单的通用框架,来解释在低维自旋能隙材料中观察到的由杂质引起的普遍低温冻结现象。