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平面金属结构中表面等离激元 - 极化激元增益的建模

Modeling surface plasmon-polariton gain in planar metallic structures.

作者信息

De Leon Israel, Berini Pierre

机构信息

School of Information Technology and Engineering, University of Ottawa, 161 Louis Pasteur, Ottawa, Ontario K1N 6N5, Canada.

出版信息

Opt Express. 2009 Oct 26;17(22):20191-202. doi: 10.1364/OE.17.020191.

Abstract

Amplification of the single-interface and long-range surface plasmon-polariton modes is studied in planar metallic structures incorporating gain media formed by Rhodamine 6G dye molecules in solution. We employ a theoretical model that accounts for the nonuniformity of the gain medium close to the metal surface due to position-dependent dipole lifetime and pump irradiance. The results of this model are used as a baseline for a comparative study against two simplified models: one neglects the position-dependent dipole lifetime while the other assumes a uniform gain medium. The discrepancies between the models are explained in terms of the mode overlap with the gain distribution near the metal. For the cases under analysis, the simplified models estimate the required pump irradiance with deviation factors that vary from 1.45 at the lossless conditions to 8 for gains near saturation. The relevance of describing properly the amount o gain interacting with the SPP mode and the role played by the dipole quantum efficiency are discussed.

摘要

在包含由罗丹明6G染料分子溶液形成的增益介质的平面金属结构中,研究了单界面和长程表面等离激元 - 极化子模式的放大。我们采用了一个理论模型,该模型考虑了由于位置相关的偶极子寿命和泵浦辐照度导致的靠近金属表面增益介质的不均匀性。该模型的结果被用作与两个简化模型进行对比研究的基线:一个忽略位置相关的偶极子寿命,另一个假设增益介质是均匀的。根据模式与金属附近增益分布的重叠情况解释了模型之间的差异。对于所分析的情况,简化模型估计所需泵浦辐照度的偏差因子在无损条件下为1.45,在增益接近饱和时为8。讨论了正确描述与表面等离激元极化子(SPP)模式相互作用的增益量以及偶极子量子效率所起作用的相关性。

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