Max Planck Institute for Solid State Research, D-70569 Stuttgart, Germany.
Phys Rev Lett. 2010 Jul 16;105(3):037207. doi: 10.1103/PhysRevLett.105.037207.
We report an inelastic-neutron-scattering and muon-spin-relaxation study of the effect of 2% spinless (Zn) impurities on the magnetic order and dynamics of YBa(2)Cu(3)O(6.6), an underdoped high-temperature superconductor that exhibits a prominent spin pseudogap in its normal state. Zn substitution induces static magnetic order at low temperatures and triggers a large-scale spectral-weight redistribution from the magnetic resonant mode at 38 meV into uniaxial, incommensurate spin excitations with energies well below the spin pseudogap. These observations indicate a competition between incommensurate magnetic order and superconductivity close to a quantum critical point. Comparison to prior data on La(2-x)Sr(x)CuO(4) suggests that this behavior is universal for the layered copper oxides and analogous to impurity-induced magnetic order in one-dimensional quantum magnets.
我们报告了一项非弹性中子散射和 muon 自旋弛豫研究,研究了 2%的无自旋(Zn)杂质对 YBa(2)Cu(3)O(6.6)的磁有序和动力学的影响,YBa(2)Cu(3)O(6.6)是一种欠掺杂的高温超导体,在正常状态下表现出明显的自旋赝能隙。Zn 取代在低温下诱导静态磁有序,并引发从 38 meV 的磁共振模式到各向异性、非共调自旋激发的大规模能谱权重再分布,能量远低于自旋赝能隙。这些观察结果表明,在接近量子临界点处存在非共调磁有序和超导之间的竞争。与 La(2-x)Sr(x)CuO(4)的先前数据进行比较表明,这种行为对于层状铜氧化物是普遍存在的,类似于一维量子磁体中的杂质诱导磁有序。