Ioffe Physical-Technical Institute RAS, 194021 St Petersburg, Russia.
J Phys Condens Matter. 2010 Jan 20;22(2):025301. doi: 10.1088/0953-8984/22/2/025301. Epub 2009 Dec 9.
The energy spectrum fine structure of triplet two-electron states in nanostructures is investigated theoretically. Spin-orbit interaction-induced terms in the effective Hamiltonian of the electron-electron interaction are derived for zinc blende lattice semiconductor systems: quantum wells and quantum dots. The effects of bulk and structural inversion asymmetry are taken into account. Simple analytical expressions describing the splittings of the two-electron states localized in a single quantum dot and in a lateral double quantum dot are derived. The spin degeneracy of triplet states is shown to be completely lifted by the spin-orbit interaction. An interplay of the conduction band spin splitting and the spin-orbit terms in the electron-electron interaction is discussed. The emission spectra of hot trions and of doubly charged excitons are calculated and are shown to reveal the fine structure of two-electron states.
本文从理论上研究了纳米结构中三重态双电子态的能谱精细结构。针对闪锌矿晶格半导体系统(量子阱和量子点),推导出了电子-电子相互作用的有效哈密顿量中由自旋轨道相互作用引起的项。考虑了体和结构反演不对称性的影响。推导出了描述单个量子点和横向双量子点中局域双电子态劈裂的简单解析表达式。自旋轨道相互作用完全消除了三重态的自旋简并。讨论了导带自旋劈裂和电子-电子相互作用中自旋轨道项的相互作用。计算了热三离子和双电荷激子的发射光谱,并表明它们揭示了双电子态的精细结构。