Van der Waals-Zeeman Institute, University of Amsterdam, Science Park 904, 1098 XH Amsterdam, The Netherlands.
Phys Rev Lett. 2011 Nov 4;107(19):198303. doi: 10.1103/PhysRevLett.107.198303.
Glasses behave as solids on experimental time scales due to their slow relaxation. Growing dynamic length scales due to cooperative motion of particles are believed to be central to this slow response. For quiescent glasses, however, the size of the cooperatively rearranging regions has never been observed to exceed a few particle diameters, and the observation of long-range correlations has remained elusive. Here, we provide direct experimental evidence of long-range correlations during the deformation of a dense colloidal glass. By imposing an external stress, we force structural rearrangements, and we identify long-range correlations in the fluctuations of microscopic strain and elucidate their scaling and spatial symmetry. The applied shear induces a transition from homogeneous to inhomogeneous flow at a critical shear rate, and we investigate the role of strain correlations in this transition.
由于其缓慢的弛豫,眼镜在实验时间尺度上表现为固体。由于粒子的协同运动而导致的不断增长的动态长度标度被认为是这种缓慢响应的核心。然而,对于静止的玻璃,协变重排区域的大小从未观察到超过几个粒子直径,并且一直难以观察到长程相关性。在这里,我们提供了在密集胶体玻璃变形过程中长程相关性的直接实验证据。通过施加外部应力,我们强制进行结构重排,并在微观应变的涨落中识别出长程相关性,并阐明了它们的标度和空间对称性。施加的剪切在临界剪切速率下引起从均匀流动到非均匀流动的转变,我们研究了应变相关性在这种转变中的作用。