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台湾中部地区粒径为 3μm、5.6μm 和 10μm 的颗粒中 Mn、Zn、Cr、Cu 和 Pb 的干沉降。

Dry deposition of Mn, Zn, Cr, Cu and Pb in particles of sizes of 3 μm, 5.6 μm and 10 μm in central Taiwan.

机构信息

Department of Safety, Health and Environmental Engineering, HungKuang University, Sha-Lu, Taichung 433, Taiwan.

出版信息

J Hazard Mater. 2012 Feb 15;203-204:158-68. doi: 10.1016/j.jhazmat.2011.11.098. Epub 2011 Dec 8.

Abstract

This investigates the concentrations of Mn, Zn, Cr, Cu, and Pb ambient air in total suspended particulates (TSPs) and dry deposition. The ratios of the calculated to measured dry deposition fluxes of ambient-air Mn, Zn, Cr, Cu and Pb at five characteristic sampling sites from 2009 to 2010 were determined using two dry deposition models. Experimental results demonstrate that the mean concentrations of metallic elements in TSPs and dry deposition were highest at the Quan-xing (industrial) sampling site, which is surrounded by various industrial factories and is in a severely polluted area. The mean seasonal concentrations of metallic elements in TSPs were highest in the winter and fall at all five sites. The analytical concentrations of metallic elements in fall and winter at these five sites were elevated in low winds. The Baklanov model yielded more accurate predictions concerning the dry deposition of metallic elements in ambient air when the sizes of the deposited particles were <5.6 μm, and the Noll and Fang model yielded better predictions when the sizes of the particles were >5.6 μm.

摘要

本研究调查了环境空气中总悬浮颗粒物(TSP)和干沉降中 Mn、Zn、Cr、Cu 和 Pb 的浓度。2009 年至 2010 年期间,在五个具有代表性的采样点使用两种干沉降模型,计算了大气中 Mn、Zn、Cr、Cu 和 Pb 的干沉降通量与实测值的比值。实验结果表明,在 Quan-xing(工业)采样点,TSP 和干沉降中金属元素的平均浓度最高,该采样点周围有各种工业工厂,处于严重污染区域。五个采样点的金属元素在冬季和秋季的平均季节浓度最高。在五个采样点中,在小风条件下,秋季和冬季金属元素的分析浓度较高。当沉积颗粒的尺寸 <5.6 μm 时,Baklanov 模型对大气中金属元素干沉降的预测更为准确,而当颗粒的尺寸 >5.6 μm 时,Noll 和 Fang 模型的预测效果更好。

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