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γ能谱法测量尼日利亚三角洲州油田环境土壤样本中的天然放射性,并评估辐射危害指数。

γ-Spectroscopy measurement of natural radioactivity and assessment of radiation hazard indices in soil samples from oil fields environment of Delta State, Nigeria.

机构信息

Department of Physics, Federal University of Petroleum Resources, Effurun, Nigeria.

出版信息

J Environ Radioact. 2012 Jul;109:64-70. doi: 10.1016/j.jenvrad.2011.10.012. Epub 2012 Feb 4.

Abstract

The analysis of naturally occurring radionuclides ((226)Ra, (232)Th and (40)K) has been carried out in soil samples collected from oil and gas field environment of Delta state, using gamma spectroscopy operated on a Canberra vertical high purity 2″×2″ NaI(TI) detector. The activity concentration of the samples ranges from 19.2 ± 5.6Bqkg(-1) to 94.2 ± 7.7Bqkg(-1) with mean value of 41.0 ± 5.0Bqkg(-1) for (226)Ra, 17.1 ± 3.0Bqkg(-1) to 47.5 ± 5.3Bqkg(-1) with mean value of 29.7 ± 4Bqkg(-1) for (232)Th and 107.0 ± 10.2Bqkg(-1) to 712.4 ± 38.9Bqkg(-1) with a mean value of 412.5 ± 20.0Bqkg(-1) for (40)K. These values obtained are well within the world range and values reported elsewhere in other countries, but are little above some countries reported average values and some part of Nigeria. The study also examined some radiation hazard indices, the mean values obtained are, 98.5 ± 12.3Bq.kg(-1), 0.8Bqkg(-1), 54.6ηGyh(-1), 0.07μSvy(-1), 0.3 and 0.4 for Radium equivalent activity (Ra(eq)), Representative level index (Iγ), Absorbed Dose rates (D), Annual Effective Dose Rates (E(ff) Dose), External Hazard Index (H(ex)) and Internal Hazard Index (H(in)) respectively. These calculated hazard indices to estimate the potential radiological health risk in soil and the dose rate associated with it are well below their permissible limit. The soil and sediments from the study area provide no excessive exposures for inhabitants and can be use as construction materials without posing any immediate radiological threat to the public. However, oil workers in the fields and host communities are cautioned against excess exposure to avoid future accumulative dose of these radiations from sludge and sediment of this area.

摘要

对来自三角洲州油气田环境的土壤样本进行了天然放射性核素 ((226)Ra、(232)Th 和 (40)K) 的分析,使用 Canberra 垂直高纯 2"×2" NaI(TI) 探测器进行了伽马光谱分析。样本的活度浓度范围为 19.2 ± 5.6Bqkg(-1) 至 94.2 ± 7.7Bqkg(-1),平均值为 41.0 ± 5.0Bqkg(-1) 用于 (226)Ra,17.1 ± 3.0Bqkg(-1) 至 47.5 ± 5.3Bqkg(-1),平均值为 29.7 ± 4Bqkg(-1) 用于 (232)Th 和 107.0 ± 10.2Bqkg(-1) 至 712.4 ± 38.9Bqkg(-1),平均值为 412.5 ± 20.0Bqkg(-1) 用于 (40)K。这些值在世界范围内和其他国家报告的其他地方都在范围内,但略高于一些国家的平均水平和尼日利亚的一些地区。该研究还检查了一些辐射危害指数,获得的平均值为 98.5 ± 12.3Bq.kg(-1)、0.8Bqkg(-1)、54.6ηGyh(-1)、0.07μSvy(-1)、0.3 和 0.4 用于镭当量活度 (Ra(eq))、代表性水平指数 (Iγ)、吸收剂量率 (D)、年有效剂量率 (E(ff)剂量)、外部危害指数 (H(ex)) 和内部危害指数 (H(in))。这些计算出的危害指数用于估计土壤中的潜在放射性健康风险及其相关剂量率,均远低于其允许限值。研究区域的土壤和沉积物不会对居民造成过度暴露,可以用作建筑材料,不会对公众造成任何即时的放射性威胁。然而,建议油田作业人员和当地社区居民避免过度暴露,以避免该地区的污泥和沉积物中这些辐射的未来累积剂量。

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