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交叉阴影图案上 InAs 量子点的成核序列。

Nucleation sequence of InAs quantum dots on cross-hatch patterns.

作者信息

Kanjanachuchai Songphol, Limwongse Teeravat

机构信息

Semiconductor Device Research Laboratory (Nanotec Center of Excellence), Department of Electrical Engineering, Faculty of Engineering, Chulalongkorn University, Bangkok 10330, Thailand.

出版信息

J Nanosci Nanotechnol. 2011 Dec;11(12):10787-91. doi: 10.1166/jnn.2011.3976.

Abstract

InAs quantum dots (QDs) are grown via molecular beam epitaxy on cross-hatch pattern (CHP) templates that result from lattice-mismatched epitaxy of In(x)Ga(1-x)As on (100)-GaAs substrates. Growth of InAs on low-(x = 0.10) and medium-(x = 0.13) mismatch CHPs with InAs thickness grading from sub- to beyond critical thickness show different stages of QD nucleation that is dictated mainly by surface steps. Tangential surface stress fields arising from the buried network of (110) misfit dislocations (MDs) at the InGaAs/GaAs interface are simulated in two dimensions and found to have a direct correlation to QD height at various locations, implying sequential QD nucleation at the surface intersection of the glide plane of dislocation T-section, cross-hatch intersection, threading dislocation, [1-10] MD line, and [110] MD line, followed by nucleation on the flat areas. Deviations from this nominal sequence is possible due to material anisotropy and are accounted for in the stress calculation by dislocation-specific scaling factors.

摘要

通过分子束外延在(100)-GaAs衬底上In(x)Ga(1-x)As晶格失配外延形成的交叉阴影图案(CHP)模板上生长InAs量子点(QD)。在低(x = 0.10)和中(x = 0.13)失配的CHP上生长InAs,InAs厚度从亚临界厚度到超过临界厚度渐变,显示出量子点成核的不同阶段,这主要由表面台阶决定。对InGaAs/GaAs界面处由(110)失配位错(MD)的掩埋网络产生的切向表面应力场进行二维模拟,发现其与不同位置的量子点高度直接相关,这意味着在位错T形截面滑移面的表面交点、交叉阴影交点、穿透位错、[1-10] MD线和[110] MD线处依次发生量子点成核,随后在平坦区域成核。由于材料各向异性,可能会偏离这个标称顺序,并且在应力计算中通过特定位错的缩放因子来考虑这些偏差。

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