Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.
Proc Natl Acad Sci U S A. 2012 Apr 3;109(14):5185-9. doi: 10.1073/pnas.1115347109. Epub 2012 Mar 19.
In carbon capture and storage (CCS), CO(2) is captured at power plants and then injected underground into reservoirs like deep saline aquifers for long-term storage. While CCS may be critical for the continued use of fossil fuels in a carbon-constrained world, the deployment of CCS has been hindered by uncertainty in geologic storage capacities and sustainable injection rates, which has contributed to the absence of concerted government policy. Here, we clarify the potential of CCS to mitigate emissions in the United States by developing a storage-capacity supply curve that, unlike current large-scale capacity estimates, is derived from the fluid mechanics of CO(2) injection and trapping and incorporates injection-rate constraints. We show that storage supply is a dynamic quantity that grows with the duration of CCS, and we interpret the lifetime of CCS as the time for which the storage supply curve exceeds the storage demand curve from CO(2) production. We show that in the United States, if CO(2) production from power generation continues to rise at recent rates, then CCS can store enough CO(2) to stabilize emissions at current levels for at least 100 y. This result suggests that the large-scale implementation of CCS is a geologically viable climate-change mitigation option in the United States over the next century.
在碳捕获与封存(CCS)中,CO2 在发电厂被捕获,然后注入地下深部盐水含水层等储层中进行长期封存。虽然CCS 对于在碳约束的世界中继续使用化石燃料可能至关重要,但由于地质封存容量和可持续注入率的不确定性,CCS 的部署受到了阻碍,这导致缺乏协调一致的政府政策。在这里,我们通过开发一种封存容量供应曲线来澄清 CCS 在美国减少排放的潜力,与当前的大规模容量估计不同,该曲线源自 CO2 注入和捕集的流体力学,并包含了注入率的限制。我们表明,封存供应是一个随 CCS 持续时间而增长的动态数量,我们将 CCS 的寿命解释为封存供应曲线超过 CO2 产量产生的封存需求曲线的时间。我们表明,在美国,如果来自发电的 CO2 产量继续以最近的速度上升,那么 CCS 可以储存足够多的 CO2,以使排放在当前水平上稳定至少 100 年。这一结果表明,在未来一个世纪,大规模实施 CCS 是美国在气候变化缓解方面的一种可行的地质选择。