Department of Physics of Complex Systems, Weizmann Institute of Science, Rehovot 76100, Israel.
Phys Rev Lett. 2012 May 18;108(20):203001. doi: 10.1103/PhysRevLett.108.203001. Epub 2012 May 16.
Recollision processes provide direct insight into the structure and dynamics of electronic wave functions. However, the strength of the process sets its basic limitations--the interaction couples numerous degrees of freedom. In this Letter we decouple the basic steps of the process and resolve the role of the ionic potential which is at the heart of a broad range of strong field phenomena. Specifically, we measure high harmonic generation from argon atoms. By manipulating the polarization of the laser field we resolve the vectorial properties of the interaction. Our study shows that the ionic core plays a significant role in all steps of the interaction. In particular, Coulomb focusing induces an angular deflection of the electrons before recombination. A complete spatiospectral analysis reveals the influence of the potential on the spatiotemporal properties of the emitted light.
再碰撞过程为研究电子波函数的结构和动力学提供了直接的途径。然而,该过程的强度设定了其基本限制——相互作用耦合了大量自由度。在这封信中,我们解耦了过程的基本步骤,并解决了离子势的作用,离子势是广泛的强场现象的核心。具体来说,我们测量了氩原子的高次谐波产生。通过操纵激光场的偏振,我们解析了相互作用的矢量特性。我们的研究表明,离子核在相互作用的所有步骤中都起着重要的作用。特别是,在复合之前,库仑聚焦会导致电子的角度偏转。完整的时空谱分析揭示了势对发射光的时空特性的影响。