Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
Phys Rev Lett. 2012 Nov 16;109(20):202506. doi: 10.1103/PhysRevLett.109.202506.
The neutron capture cross section of (235)U was measured for the neutron incident energy region between 4 eV and 1 MeV at the DANCE facility at the Los Alamos Neutron Science Center with an unprecedented accuracy of 2-3% at 1 keV. The new methodology combined three independent measurements. In the main experiment, a thick actinide sample was used to determine neutron capture and neutron-induced fission rates simultaneously. In the second measurement, a fission tagging detector was used with a thin actinide sample and detailed characteristics of the prompt-fission gamma rays were obtained. In the third measurement, the neutron scattering background was characterized using a sample of (208)Pb. The relative capture cross section was obtained from the experiment with the thick (235)U sample using a ratio method after the subtraction of the fission and neutron scattering backgrounds. Our result indicates errors that are as large as 30% in the 0.5-2.5 keV region, in the current knowledge of neutron capture as embodied in major nuclear data evaluations. Future modifications of these databases using the improved precision data given herein will have significant impacts in neutronics calculations for a variety of nuclear technologies.
(235)U 的中子俘获截面在洛斯阿拉莫斯国家实验室的 DANCE 设施中进行了测量,测量能区为 4 eV 到 1 MeV,在 1 keV 处精度达到了前所未有的 2-3%。新方法结合了三种独立的测量方法。在主实验中,使用厚的锕系元素样品同时确定了中子俘获和中子诱发裂变的速率。在第二个测量中,使用薄的锕系元素样品和裂变标记探测器,并获得了瞬发裂变伽马射线的详细特征。在第三个测量中,使用 (208)Pb 样品对中子散射背景进行了表征。相对俘获截面是从厚 (235)U 样品的实验中通过减去裂变和中子散射背景后用比值法得到的。我们的结果表明,在当前主要核数据评估中体现的 0.5-2.5 keV 能区的中子俘获知识中,存在高达 30%的误差。使用本文提供的改进精度数据对这些数据库进行未来的修正,将对各种核技术的中子学计算产生重大影响。