Wigner Research Centre for Physics, Konkoly-Thege M. út 29-33, 1121 Budapest, Hungary.
Nano Lett. 2013 Feb 13;13(2):674-8. doi: 10.1021/nl304365e. Epub 2013 Jan 25.
We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become strongly accelerated within the evanescent fields of the plasmonic nanoparticles and escape along straight trajectories with orientations governed by the particle geometry. These results establish plasmonic nanoparticles as versatile ultrafast, nanoscopic sources of electrons.
我们展示了从定制的金属纳米粒子中超快产生电子,并通过比较共振和非共振粒子以及不同的粒子几何形状,揭示了等离子体场增强在这一过程中的作用。我们发现,电子在等离子体纳米粒子的消逝场中被强烈加速,并沿着由粒子几何形状决定的方向沿直线轨迹逃逸。这些结果确立了等离子体纳米粒子作为多功能超快纳米尺度电子源。