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软 X 射线角分辨光电子能谱学设施在 SLS 的 ADRESS 光束线上:概念、技术实现和科学应用。

Soft-X-ray ARPES facility at the ADRESS beamline of the SLS: concepts, technical realisation and scientific applications.

机构信息

Swiss Light Source, Paul Scherrer Institute, CH-5232 Villigen-PSI, Switzerland.

出版信息

J Synchrotron Radiat. 2014 Jan;21(Pt 1):32-44. doi: 10.1107/S1600577513019085. Epub 2013 Nov 7.

Abstract

Soft-X-ray angle-resolved photoelectron spectroscopy (ARPES) with photon energies around 1 keV combines the momentum space resolution with increasing probing depth. The concepts and technical realisation of the new soft-X-ray ARPES endstation at the ADRESS beamline of SLS are described. The experimental geometry of the endstation is characterized by grazing X-ray incidence on the sample to increase the photoyield and vertical orientation of the measurement plane. The vacuum chambers adopt a radial layout allowing most efficient sample transfer. High accuracy of the angular resolution is ensured by alignment strategies focused on precise matching of the X-ray beam and optical axis of the analyzer. The high photon flux of up to 10(13) photons s(-1) (0.01% bandwidth)(-1) delivered by the beamline combined with the optimized experimental geometry break through the dramatic loss of the valence band photoexcitation cross section at soft-X-ray energies. ARPES images with energy resolution up to a few tens of meV are typically acquired on the time scale of minutes. A few application examples illustrate the power of our advanced soft-X-ray ARPES instrumentation to explore the electronic structure of bulk crystals with resolution in three-dimensional momentum, access buried heterostructures and study elemental composition of the valence states using resonant excitation.

摘要

软 X 射线角分辨光电子能谱(ARPES),其光子能量约为 1keV,将动量空间分辨率与增加的探测深度相结合。本文描述了 SLS 的 ADRESS 光束线新的软 X 射线 ARPES 端站的概念和技术实现。端站的实验几何结构的特点是掠射 X 射线入射到样品上,以增加光产率和测量平面的垂直取向。真空室采用径向布局,允许最有效地进行样品转移。通过聚焦于精确匹配 X 射线束和分析器光轴的对准策略,确保了角分辨率的高精度。高达 10(13) 光子 s(-1)(0.01%带宽)(-1)的光束线提供的高光子通量与优化的实验几何结构相结合,突破了软 X 射线能量下价带光激发截面的急剧损失。通常在几分钟的时间尺度内,就能获得能量分辨率高达几十毫电子伏特的 ARPES 图像。一些应用实例说明了我们先进的软 X 射线 ARPES 仪器的强大功能,它可以在三维动量分辨率下探索体晶体的电子结构,探测掩埋异质结构,并使用共振激发研究价态的元素组成。

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