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热等离子体学:在单根纳米线中量化等离子体加热。

Thermoplasmonics: quantifying plasmonic heating in single nanowires.

机构信息

Department of Physics and Astronomy, Rice University , Houston, Texas 77005, United States.

出版信息

Nano Lett. 2014 Feb 12;14(2):499-503. doi: 10.1021/nl403510u. Epub 2014 Jan 9.

Abstract

Plasmonic absorption of light can lead to significant local heating in metallic nanostructures, an effect that defines the subfield of thermoplasmonics and has been leveraged in diverse applications from biomedical technology to optoelectronics. Quantitatively characterizing the resulting local temperature increase can be very challenging in isolated nanostructures. By measuring the optically induced change in resistance of metal nanowires with a transverse plasmon mode, we quantitatively determine the temperature increase in single nanostructures with the dependence on incident polarization clearly revealing the plasmonic heating mechanism. Computational modeling explains the resonant and nonresonant contributions to the optical heating and the dominant pathways for thermal transport. These results, obtained by combining electronic and optical measurements, place a bound on the role of optical heating in prior experiments and suggest design guidelines for engineered structures meant to leverage such effects.

摘要

光的等离子体吸收会导致金属纳米结构中产生显著的局部加热,这种效应定义了热等离子体学的子领域,并在从生物医学技术到光电子学的各种应用中得到了利用。在孤立的纳米结构中,定量描述由此产生的局部温度升高是非常具有挑战性的。通过测量具有横向等离子体模式的金属纳米线的光诱导电阻变化,我们定量确定了单个纳米结构中的温度升高,其对入射偏振的依赖性清楚地揭示了等离子体加热机制。计算模型解释了光学加热的共振和非共振贡献以及热传输的主要途径。这些通过结合电子和光学测量获得的结果,对先前实验中光学加热的作用进行了限制,并为旨在利用这种效应的工程结构提供了设计指南。

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