Department of Materials Science and Engineering, ‡Department of Chemistry, and §Department of Medicine, Northwestern University , Evanston, Illinois 60208, United States.
ACS Nano. 2014 Feb 25;8(2):1102-20. doi: 10.1021/nn500064s. Epub 2014 Jan 31.
With advances in exfoliation and synthetic techniques, atomically thin films of semiconducting transition metal dichalcogenides have recently been isolated and characterized. Their two-dimensional structure, coupled with a direct band gap in the visible portion of the electromagnetic spectrum, suggests suitability for digital electronics and optoelectronics. Toward that end, several classes of high-performance devices have been reported along with significant progress in understanding their physical properties. Here, we present a review of the architecture, operating principles, and physics of electronic and optoelectronic devices based on ultrathin transition metal dichalcogenide semiconductors. By critically assessing and comparing the performance of these devices with competing technologies, the merits and shortcomings of this emerging class of electronic materials are identified, thereby providing a roadmap for future development.
随着剥离和合成技术的进步,最近已经分离并表征出了原子层厚度的半导体过渡金属二卤化物薄膜。它们的二维结构,加上在电磁光谱可见光部分的直接带隙,表明它们适合用于数字电子学和光电子学。为此,已经报道了几类高性能器件,并在理解其物理性质方面取得了重大进展。在这里,我们对基于超薄过渡金属二卤化物半导体的电子和光电子器件的架构、工作原理和物理特性进行了综述。通过批判性地评估和比较这些器件与竞争技术的性能,确定了这种新兴电子材料类别的优点和缺点,从而为未来的发展提供了路线图。