Key Laboratory of Nuclear Radiation and Nuclear Energy Technology, Institute of High Enegy Physics, Chinese Academy of Sciences, Beijing, 100049, China.
Adv Mater. 2014 Dec 10;26(46):7807-48. doi: 10.1002/adma.201304323. Epub 2014 Aug 28.
Synchrotron radiation (SR) based techniques have been utilized with increasing frequency in the past decade to explore the brilliant and challenging sciences of actinide-based materials. This trend is partially driven by the basic needs for multi-scale actinide speciation and bonding information and also the realistic needs for nuclear energy research. In this review, recent research progresses on actinide related materials by means of various SR techniques were selectively highlighted and summarized, with the emphasis on X-ray absorption spectroscopy, X-ray diffraction and scattering spectroscopy, which are powerful tools to characterize actinide materials. In addition, advanced SR techniques for exploring future advanced nuclear fuel cycles dealing with actinides are illustrated as well.
过去十年中,基于同步加速器辐射(SR)的技术越来越频繁地被用于探索基于锕系元素的材料这一精彩而具有挑战性的科学领域。这种趋势的部分原因是对锕系元素多尺度形态和键合信息的基本需求,以及对核能研究的实际需求。在这篇综述中,我们有选择性地突出并总结了各种同步辐射技术在研究与锕系元素相关材料方面的最新进展,重点介绍了X 射线吸收光谱学、X 射线衍射和散射光谱学,这些都是研究锕系元素材料的有力工具。此外,我们还介绍了用于探索未来涉及锕系元素的先进核燃料循环的先进同步辐射技术。