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GaAs/InGaAs/GaAs纳米线芯-多壳量子阱异质结构的制备及其光学性质

Fabrication and optical properties of GaAs/InGaAs/GaAs nanowire core-multishell quantum well heterostructures.

作者信息

Yan Xin, Zhang Xia, Li Junshuai, Wu Yao, Cui Jiangong, Ren Xiaomin

机构信息

State Key Laboratory of Information Photonics and Optical Communications, Beijing University of Posts and Telecommunications, Beijing 100876, China.

出版信息

Nanoscale. 2015 Jan 21;7(3):1110-5. doi: 10.1039/c4nr05486e.

Abstract

GaAs/InGaAs/GaAs nanowire core-multishell heterostructures with a strained radial In0.2Ga0.8As quantum well were fabricated by metal organic chemical vapor deposition. The quantum well exhibits a dislocation-free phase-pure zinc-blende structure. Low-temperature photoluminescence spectra of a single nanowire exhibit distinct resonant peaks in the range from 880 to 1000 nm, corresponding to the longitudinal modes of a Fabry-Pérot cavity. This suggests a decoupling of the gain medium and resonant cavity so that the quantum well provides the gain while the nanowire acts as the cavity. The resonant modes were observed at temperatures up to 240 K, exhibiting high power- and temperature-stability. The modes were blueshifted while decreasing the quantum well thickness due to enhanced quantum confinement. The results make the GaAs-based nanowire/quantum well hybrid structure promising for wavelength-tunable near-infrared nanolasers.

摘要

通过金属有机化学气相沉积法制备了具有应变径向In0.2Ga0.8As量子阱的GaAs/InGaAs/GaAs纳米线芯-多壳异质结构。该量子阱呈现出无位错的纯闪锌矿结构。单根纳米线的低温光致发光光谱在880至1000nm范围内呈现出明显的共振峰,对应于法布里-珀罗腔的纵向模式。这表明增益介质和谐振腔发生了解耦,使得量子阱提供增益而纳米线充当腔。在高达240K的温度下观察到了共振模式,表现出高功率和温度稳定性。由于量子限制增强,在减小量子阱厚度时模式发生蓝移。这些结果使得基于GaAs的纳米线/量子阱混合结构有望用于波长可调谐近红外纳米激光器。

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