Persson Olof, Webb James L, Dick Kimberly A, Thelander Claes, Mikkelsen Anders, Timm Rainer
§Center for Analysis and Synthesis, Lund University, Box 124, 221 00 Lund, Sweden.
Nano Lett. 2015 Jun 10;15(6):3684-91. doi: 10.1021/acs.nanolett.5b00898. Epub 2015 May 5.
Using a scanning tunneling and atomic force microscope combined with in-vacuum atomic hydrogen cleaning we demonstrate stable scanning tunneling spectroscopy (STS) with nanoscale resolution on electrically active nanowire devices in the common lateral configuration. We use this method to map out the surface density of states on both the GaSb and InAs segments of GaSb-InAs Esaki diodes as well as the transition region between the two segments. Generally the surface shows small bandgaps centered around the Fermi level, which is attributed to a thin multielement surface layer, except in the diode transition region where we observe a sudden broadening of the bandgap. By applying a bias to the nanowire we find that the STS spectra shift according to the local nanoscale potential drop inside the wire. Importantly, this shows that we have a nanoscale probe with which we can infer both surface electronic structure and the local potential inside the nanowire and we can connect this information directly to the performance of the imaged device.
利用扫描隧道显微镜和原子力显微镜,并结合真空原子氢清洗技术,我们展示了在常见横向配置的电活性纳米线器件上具有纳米级分辨率的稳定扫描隧道谱(STS)。我们使用这种方法来绘制GaSb-InAs埃萨基二极管的GaSb和InAs段以及两段之间的过渡区域的表面态密度。一般来说,除了在二极管过渡区域观察到带隙突然变宽外,表面在费米能级附近显示出小的带隙,这归因于一个薄的多元素表面层。通过向纳米线施加偏压,我们发现STS谱会根据纳米线内部的局部纳米级电势降而发生移动。重要的是,这表明我们拥有一个纳米级探针,利用它我们可以推断纳米线的表面电子结构和局部电势,并且我们可以将这些信息直接与成像器件的性能联系起来。