Department of Mechanical Engineering, Colorado State University , Fort Collins, Colorado 80523, United States.
The Energy Institute, Colorado State University , Fort Collins, Colorado 80523, United States.
Environ Sci Technol. 2015 Sep 1;49(17):10718-27. doi: 10.1021/acs.est.5b02275. Epub 2015 Aug 18.
New facility-level methane (CH4) emissions measurements obtained from 114 natural gas gathering facilities and 16 processing plants in 13 U.S. states were combined with facility counts obtained from state and national databases in a Monte Carlo simulation to estimate CH4 emissions from U.S. natural gas gathering and processing operations. Total annual CH4 emissions of 2421 (+245/-237) Gg were estimated for all U.S. gathering and processing operations, which represents a CH4 loss rate of 0.47% (±0.05%) when normalized by 2012 CH4 production. Over 90% of those emissions were attributed to normal operation of gathering facilities (1697 +189/-185 Gg) and processing plants (506 +55/-52 Gg), with the balance attributed to gathering pipelines and processing plant routine maintenance and upsets. The median CH4 emissions estimate for processing plants is a factor of 1.7 lower than the 2012 EPA Greenhouse Gas Inventory (GHGI) estimate, with the difference due largely to fewer reciprocating compressors, and a factor of 3.0 higher than that reported under the EPA Greenhouse Gas Reporting Program. Since gathering operations are currently embedded within the production segment of the EPA GHGI, direct comparison to our results is complicated. However, the study results suggest that CH4 emissions from gathering are substantially higher than the current EPA GHGI estimate and are equivalent to 30% of the total net CH4 emissions in the natural gas systems GHGI. Because CH4 emissions from most gathering facilities are not reported under the current rule and not all source categories are reported for processing plants, the total CH4 emissions from gathering and processing reported under the EPA GHGRP (180 Gg) represents only 14% of that tabulated in the EPA GHGI and 7% of that predicted from this study.
从美国 13 个州的 114 个天然气收集设施和 16 个处理厂获得的新的设施层面甲烷(CH4)排放测量值,与从州和国家数据库获得的设施计数相结合,在蒙特卡罗模拟中进行估算,以估计美国天然气收集和处理作业的 CH4 排放量。所有美国收集和处理作业的年总 CH4 排放量估计为 2421(+245/-237)Gg,这表示在 2012 年 CH4 产量的基础上归一化时,CH4 损失率为 0.47%(±0.05%)。这些排放中有超过 90%归因于收集设施(1697 +189/-185 Gg)和处理厂(506 +55/-52 Gg)的正常运行,其余部分归因于收集管道和处理厂的常规维护和故障。处理厂的 CH4 排放量中位数估计值比 2012 年 EPA 温室气体清单(GHGI)的估计值低 1.7 倍,这主要是由于往复式压缩机较少,以及比 EPA 温室气体报告计划报告的值高 3.0 倍。由于收集作业目前嵌入在 EPA GHGI 的生产部分中,因此与我们的结果进行直接比较很复杂。然而,研究结果表明,收集过程中的 CH4 排放量远远高于当前 EPA GHGI 的估计值,相当于天然气系统 GHGI 中总净 CH4 排放量的 30%。由于目前的规定没有报告大多数收集设施的 CH4 排放量,并且没有报告处理厂的所有源类别,因此 EPA GHGRP 报告的收集和处理总 CH4 排放量(180 Gg)仅占 EPA GHGI 中列出的排放量的 14%,占本研究预测值的 7%。