Li Baochuan, Wang Nanping, Wan Jianhua, Xiong Shengqing, Liu Hongtao, Li Shijun, Zhao Rong
Geo-detection Laboratory, Ministry of Education, China University of Geosciences, China; School of Geophysics and Information Technology, China University of Geosciences (Beijing), 29 Xueyuan Road, Beijing, 100083, China.
Geo-detection Laboratory, Ministry of Education, China University of Geosciences, China; School of Geophysics and Information Technology, China University of Geosciences (Beijing), 29 Xueyuan Road, Beijing, 100083, China.
J Environ Radioact. 2016 Jan;151 Pt 1:304-310. doi: 10.1016/j.jenvrad.2015.10.027. Epub 2015 Nov 8.
An in-situ gamma-ray spectrometer survey with a scintillation detector of NaI(Tl) (Φ75 mm × 75 mm) was carried out in the Baotou and Bayan Obo Districts in order to estimate the levels of natural radionuclides near rare-earth (RE) tailings dams. In the RE tailings dam of Baotou, the mean concentrations of (238)U and (232)Th were 3.0 ± 1.0 mg/kg (range: 1.9-4.6 mg/kg) and 321 ± 31 mg/kg (range: 294-355 mg/kg), respectively. In the Bayan Obo tailings dam, the mean concentrations of (238)U and (232)Th were 5.7 ± 0.5 mg/kg (range: 5.3-6.1 mg/kg) and 276 ± 0.5 mg/kg (range: 275.5-276.3 mg/kg), respectively. The average (232)Th concentrations in the mining areas of the Bayan Obo Mine and the living areas of the Bayan Obo Town were 18.7 ± 7.5 and 26.2 ± 9.1 mg/kg, respectively. The (232)Th concentration recorded in the tailings dams was much higher than the global average (7.44 mg/kg). Our investigation shows that the (232)Th concentration in the tailings in the Baotou dam was 34.6 times greater than that in the local soil (in Guyang County); the average concentrations of (232)Th in the soil in the Baotou District and Bayan Obo Districts were about 1.35 and 2.82 times greater, respectively, than that in the soil in Guyang County. Based on our results, the highest estimated effective dose due to gamma irradiation was 1.15 mSv per year, estimated from the data observed in the Baotou tailings dams. The results of this preliminary study indicate the potential importance of radioactivity in RE tailings dams and that remedial measures may be required.
为了估算稀土尾矿坝附近天然放射性核素的水平,使用碘化钠(铊)闪烁探测器(Φ75毫米×75毫米)在包头和白云鄂博地区进行了原位伽马射线能谱测量。在包头的稀土尾矿坝中,²³⁸U和²³²Th的平均浓度分别为3.0±1.0毫克/千克(范围:1.9 - 4.6毫克/千克)和321±31毫克/千克(范围:294 - 355毫克/千克)。在白云鄂博尾矿坝中,²³⁸U和²³²Th的平均浓度分别为5.7±0.5毫克/千克(范围:5.3 - 6.1毫克/千克)和276±0.5毫克/千克(范围:275.5 - 276.3毫克/千克)。白云鄂博矿矿区和白云鄂博镇生活区的²³²Th平均浓度分别为18.7±7.5和26.2±9.1毫克/千克。尾矿坝中记录的²³²Th浓度远高于全球平均水平(7.44毫克/千克)。我们的调查表明,包头尾矿坝中尾矿的²³²Th浓度比当地土壤(固阳县)中的浓度高34.6倍;包头地区和白云鄂博地区土壤中²³²Th的平均浓度分别比固阳县土壤中的浓度高约1.35倍和2.82倍。根据我们的结果,从包头尾矿坝观测数据估算,因伽马辐射导致的最高有效剂量估计为每年1.15毫希沃特。这项初步研究结果表明了稀土尾矿坝中放射性的潜在重要性,可能需要采取补救措施。