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采用聚氨酯泡沫塑料填充的生物滴滤过滤法去除 2-丁氧基乙醇气态排放物。

Removal of 2-butoxyethanol gaseous emissions by biotrickling filtration packed with polyurethane foam.

机构信息

Research Group GI(2)AM, Department of Chemical Engineering, Universitat de València, Av. de la Universitat s/n, 46100 Burjassot, Spain.

Research Group ALR, Department of Biological Waste Air Purification, Institute of Sanitary Engineering, Water Quality and Solid Waste Management, University of Stuttgart, Bandtäle 2, 70569 Stuttgart, Germany.

出版信息

N Biotechnol. 2016 Mar 25;33(2):263-72. doi: 10.1016/j.nbt.2015.11.006. Epub 2015 Nov 17.

Abstract

The removal of 2-butoxyethanol from gaseous emissions was studied using two biotrickling filters (BTF1 and BTF2) packed with polyurethane foam. Two different inoculum sources were used: a pure culture of Pseudomonas sp. BOE200 (BTF1) and activated sludge from a municipal wastewater treatment plant (BTF2). The bioreactors were operated at inlet loads (ILs) of 130 and 195 g m(-3) hour(-1) and at an empty bed residence time (EBRT) of 12.5s. Under an IL of ∼130 g m(-3) hour(-1), BTF1 presented higher elimination capacities (ECs) than BTF2, with average values of 106±7 and 68±8 g m(-3) hour(-1), respectively. However, differences in ECs between BTFs were decreased by reducing the irrigation intervals from 1 min every 12 min to 1 min every 2 hours in BTF2. Average values of EC were 111±25 and 90±7 g m(-3) hour(-1) for BTF1 and BTF2, respectively, when working at an IL of ∼195 g m(-3) hour(-1). Microbial analysis revealed a significant shift in the microbial community of BTF1 inoculated with Pseudomonas sp. BOE200. At the end of the experiment, the species Microbacterium sp., Chryseobacterium sp., Acinetobacter sp., Pseudomonas sp. and Mycobacterium sp. were detected. In BTF2 inoculated with activated sludge, the denaturing gradient gel electrophoresis (DGGE) technique showed a diverse microbial community including species that was able to use 2-butoxyethanol as its carbon source, such as Pseudomonas aeruginosa and Pseudomonas putida as representative species. Although BTF1 inoculated with Pseudomonas sp. BOE200 and higher gas velocity (probably greater gas/liquid mass transfer rate) showed a slight improvement in performance, the use of activated sludge as inoculum seems to be a more feasible option for the industrial application of this technology.

摘要

采用聚氨酯泡沫作为填料,利用两个生物滴滤塔(BTF1 和 BTF2)研究了从气态排放物中去除 2-丁氧基乙醇。使用了两种不同的接种源:一种是纯 Pseudomonas sp. BOE200 培养物(BTF1),另一种是城市污水处理厂的活性污泥(BTF2)。生物反应器的入口负荷(IL)分别为 130 和 195 g m(-3) 小时(-1),空床停留时间(EBRT)为 12.5 s。在 IL 约为 130 g m(-3) 小时(-1)时,BTF1 的去除效率(EC)高于 BTF2,平均值分别为 106±7 和 68±8 g m(-3) 小时(-1)。然而,通过将 BTF2 的灌溉间隔从 12 min 缩短至 2 h,BTF1 和 BTF2 的 EC 差异减小。当 IL 约为 195 g m(-3) 小时(-1)时,BTF1 和 BTF2 的 EC 平均值分别为 111±25 和 90±7 g m(-3) 小时(-1)。微生物分析表明,接种 Pseudomonas sp. BOE200 的 BTF1 的微生物群落发生了显著变化。实验结束时,检测到 Microbacterium sp.、Chryseobacterium sp.、Acinetobacter sp.、Pseudomonas sp. 和 Mycobacterium sp. 等物种。接种活性污泥的 BTF2 中,变性梯度凝胶电泳(DGGE)技术显示出一个多样化的微生物群落,包括能够将 2-丁氧基乙醇作为碳源的物种,如 Pseudomonas aeruginosa 和 Pseudomonas putida 等代表物种。尽管接种 Pseudomonas sp. BOE200 的 BTF1 和更高的气体速度(可能具有更大的气/液传质速率)在性能上略有提高,但使用活性污泥作为接种物似乎是该技术工业应用的更可行选择。

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