Mao Linqiang, Gao Bingying, Deng Ning, Liu Lu, Cui Hao
State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University, Nanjing 210046, PR China.
College of Chemistry and Chemical Engineering, Hunan Normal University, Changsha 410081, PR China.
Chemosphere. 2016 Feb;145:1-9. doi: 10.1016/j.chemosphere.2015.11.053. Epub 2015 Dec 1.
The oxidation behavior of Cr(III) during the thermal treatment of chromium hydroxide in the presence of alkali and alkaline earth metal chlorides (NaCl, KCl, MgCl2, and CaCl2) was investigated. The amounts of Cr(III) oxidized at various temperatures and heating times were determined, and the Cr-containing species in the residues were characterized. During the transformation of chromium hydroxide to Cr2O3 at 300 °C approximately 5% of the Cr(III) was oxidized to form intermediate compounds containing Cr(VI) (i.e., CrO3), but these intermediates were reduced to Cr2O3 when the temperature was above 400 °C. Alkali and alkaline earth metals significantly promoted the oxidation of Cr(III) during the thermal drying process. Two pathways were involved in the influences the alkali and alkaline earth metals had on the formation of Cr(VI). In pathway I, the alkali and alkaline earth metals were found to act as electron transfer agents and to interfere with the dehydration process, causing more intermediate Cr(VI)-containing compounds (which were identified as being CrO3 and Cr5O12) to be formed. The reduction of intermediate compounds to Cr2O3 was also found to be hindered in pathway I. In pathway II, the alkali and alkaline earth metals were found to contribute to the oxidation of Cr(III) to form chromates. The results showed that the presence of alkali and alkaline earth metals significantly increases the degree to which Cr(III) is oxidized during the thermal drying of chromium-containing sludge.
研究了在碱金属和碱土金属氯化物(NaCl、KCl、MgCl₂和CaCl₂)存在下氢氧化铬热处理过程中Cr(III)的氧化行为。测定了不同温度和加热时间下被氧化的Cr(III)的量,并对残渣中含铬物种进行了表征。在300℃氢氧化铬向Cr₂O₃的转变过程中,约5%的Cr(III)被氧化形成含Cr(VI)的中间化合物(即CrO₃),但当温度高于400℃时,这些中间产物被还原为Cr₂O₃。碱金属和碱土金属在热干燥过程中显著促进了Cr(III)的氧化。碱金属和碱土金属对Cr(VI)形成的影响涉及两条途径。在途径I中,发现碱金属和碱土金属充当电子转移剂并干扰脱水过程,导致形成更多含Cr(VI)的中间化合物(经鉴定为CrO₃和Cr₅O₁₂)。在途径I中还发现中间化合物向Cr₂O₃的还原也受到阻碍。在途径II中,发现碱金属和碱土金属有助于将Cr(III)氧化形成铬酸盐。结果表明,碱金属和碱土金属的存在显著提高了含铬污泥热干燥过程中Cr(III)的氧化程度。