Wolf Daniel, Rodriguez Luis A, Béché Armand, Javon Elsa, Serrano Luis, Magen Cesar, Gatel Christophe, Lubk Axel, Lichte Hannes, Bals Sara, Van Tendeloo Gustaaf, Fernández-Pacheco Amalio, De Teresa José M, Snoeck Etienne
Triebenberg Laboratory, Institute of Structural Physics, Technische Universität Dresden , 01062 Dresden, Saxony, Germany.
Laboratorio de Microscopías Avanzadas (LMA), Instituto de Nanociencia de Aragón (INA), Universidad de Zaragoza, 50018 Zaragoza, Spain; Transpyrenean Associated Laboratory for Electron Microscopy (TALEM), CEMES INA CNRS-Universidad de Zaragoza, 31400 Toulouse, France; CEMES-CNRS 29, rue Jeanne Marvig, B.P. 94347 F-31055, Toulouse Cedex, France.
Chem Mater. 2015 Oct 13;27(19):6771-6778. doi: 10.1021/acs.chemmater.5b02723. Epub 2015 Sep 8.
The investigation of three-dimensional (3D) ferromagnetic nanoscale materials constitutes one of the key research areas of the current magnetism roadmap and carries great potential to impact areas such as data storage, sensing, and biomagnetism. The properties of such nanostructures are closely connected with their 3D magnetic nanostructure, making their determination highly valuable. Up to now, quantitative 3D maps providing both the internal magnetic and electric configuration of the same specimen with high spatial resolution are missing. Here, we demonstrate the quantitative 3D reconstruction of the dominant axial component of the magnetic induction and electrostatic potential within a cobalt nanowire (NW) of 100 nm in diameter with spatial resolution below 10 nm by applying electron holographic tomography. The tomogram was obtained using a dedicated TEM sample holder for acquisition, in combination with advanced alignment and tomographic reconstruction routines. The powerful approach presented here is widely applicable to a broad range of 3D magnetic nanostructures and may trigger the progress of novel spintronic nonplanar nanodevices.
对三维(3D)铁磁纳米级材料的研究是当前磁学路线图的关键研究领域之一,在数据存储、传感和生物磁学等领域具有巨大的潜在影响力。此类纳米结构的特性与其3D磁性纳米结构密切相关,因此对其进行测定具有很高的价值。到目前为止,缺少能够以高空间分辨率提供同一标本内部磁配置和电配置的定量3D图谱。在此,我们通过应用电子全息断层扫描技术,展示了对直径为100 nm的钴纳米线(NW)内磁感应强度和静电势的主要轴向分量进行定量3D重建,空间分辨率低于10 nm。断层图像是使用专门的透射电子显微镜(TEM)样品架进行采集,并结合先进的对准和断层重建程序获得的。本文提出的强大方法广泛适用于各种3D磁性纳米结构,并可能推动新型自旋电子非平面纳米器件的发展。