Institute of Super-microstructure and Ultrafast Process in Advanced Materials (ISUPAM), School of Physics and Electronics, Central South University, Changsha, Hunan 410083, PR China.
Nanoscale. 2016 Aug 14;8(30):14580-6. doi: 10.1039/c6nr02915a. Epub 2016 Jul 18.
CdS heterostructure nanomaterials are attractive for their potential applications in integrated optoelectronic devices. Herein, the high-quality CdS/CdS:SnS2 superlattice nanowires were synthesized through a micro-environmental controlled co-evaporation technique, which shows periodic emission properties and that their structures are periodic and alternating. For the first time, we demonstrate the fabrication of high-performance ultraviolet photodetectors using unique CdS/CdS:SnS2 superlattice nanowires. The optoelectronic properties of the photodetectors were studied and compared to those devices based on pure CdS nanowires. The as-fabricated photodetectors (under 365 nm) based on CdS/CdS:SnS2 superlattice nanowires showed a high photocurrent to dark current ratio of 10(5), a large photoresponsivity of 2.5 × 10(3) A W(-1), a fast response time of 10 ms and an excellent external quantum efficiency of 8.6 × 10(5) at room temperature, which shows better performance than pure CdS nanowires photodetectors. The results indicate that CdS/CdS:SnS2 superlattice nanowires are very promising potential candidates in nanoscale electronic and optoelectronic devices.
CdS 异质结构纳米材料因其在集成光电器件中的潜在应用而备受关注。本文通过微环境控制共蒸发技术合成了高质量的 CdS/CdS:SnS2 超晶格纳米线,其具有周期性发射特性,结构呈周期性交替排列。本文首次利用独特的 CdS/CdS:SnS2 超晶格纳米线制备了高性能的紫外光探测器。研究了光探测器的光电性能,并与基于纯 CdS 纳米线的器件进行了比较。所制备的基于 CdS/CdS:SnS2 超晶格纳米线的光探测器(在 365nm 下)表现出高光电流与暗电流比为 10(5)、大光响应度为 2.5×10(3)A W(-1)、快速响应时间为 10ms 和室温下的优异外量子效率为 8.6×10(5),其性能优于纯 CdS 纳米线光探测器。结果表明,CdS/CdS:SnS2 超晶格纳米线是纳米尺度电子和光电器件中有前途的候选材料。