Desideri Donatella, Cantaluppi Chiara, Ceccotto Federica, Meli Maria Assunta, Roselli Carla, Feduzi Laura
*Biomolecular Sciences Department, Urbino University "Carlo Bo," P.zza Rinascimento 6, 61029 Urbino, Italy; †CNR-IENI, Corso Stati Uniti 4, 35127 Padova, Italy.
Health Phys. 2016 Sep;111(3):256-64. doi: 10.1097/HP.0000000000000526.
Natural radionuclides and Cs were determined by alpha (U, U, Th,Po,Th, and Th) and gamma spectrometry (Cs, K, Ra, Pb, and Ra via Ac) in 14 dried seaweeds commercialized for human nutrition in Italy. The study was carried out in order to provide information on the concentrations of natural and artificial radionuclides. Cesium-137 (Cs) concentrations in all analyzed samples were always <2.0 Bq kg (dry weight), while the naturally occurring radionuclide concentrations were detectable in all the samples and significantly different in the analyzed seaweeds. Potassium-40 (K) showed a mean activity of 894 Bq kg with a range of 14.1-3,256 Bq kg. The mean of activity for Po was 5.1 Bq kg with a range of 1.5-13.6 Bq kg. The mean of activity for Pb was 8.9 Bq kg with a range of 2.9-25.7 Bq kg. The mean of U and Ra activity concentration was 4.7 and 8.4 Bq kg with a range of 0.1-27.7 and 3.2-24.6 Bq kg, respectively. The mean activity concentrations for Th, Th, and Ra were 0.69, 3.0, and 6.6 Bq kg with ranges of 0.05-3.39, 0.24-15.7, and 0.5-35.6 Bq kg, respectively. Radionuclide activity concentrations were within ranges reported in the scientific literature. The committed effective dose due to all the radionuclides analyzed, from ingestion of 1 kg y of seaweeds, accounts for 0.66% of the natural radiation exposure in Italy.
采用α能谱法(测定U、U、Th、Po、Th和Th)和γ能谱法(通过Ac测定Cs、K、Ra、Pb和Ra),对意大利市场上作为人类营养食品销售的14种干海藻中的天然放射性核素和Cs进行了测定。开展该研究是为了提供有关天然和人工放射性核素浓度的信息。所有分析样品中的铯 - 137(Cs)浓度均始终<2.0 Bq/kg(干重),而天然存在的放射性核素浓度在所有样品中均可检测到,且在所分析的海藻中存在显著差异。钾 - 40(K)的平均活度为894 Bq/kg,范围为14.1 - 3256 Bq/kg。钋(Po)的平均活度为5.1 Bq/kg,范围为1.5 - 13.6 Bq/kg。铅(Pb)的平均活度为8.9 Bq/kg,范围为2.9 - 25.7 Bq/kg。U和Ra的活度浓度平均值分别为4.7和8.4 Bq/kg,范围分别为0.1 - 27.7和3.2 - 24.6 Bq/kg。Th、Th和Ra的平均活度浓度分别为0.69、3.0和6.6 Bq/kg,范围分别为0.05 - 3.39、0.24 - 15.7和0.5 - 35.6 Bq/kg。放射性核素活度浓度在科学文献报道的范围内。因摄入1 kg/年的海藻而受到的所有分析放射性核素所致的待积有效剂量,占意大利天然辐射暴露量的0.66%。