Grünwald P, Aßmann M, Heckötter J, Fröhlich D, Bayer M, Stolz H, Scheel S
Institut für Physik, Universität Rostock, Albert-Einstein-Strasse 23, D-18059 Rostock, Germany.
Experimentelle Physik 2, Technische Universität Dortmund, D-44221 Dortmund, Germany.
Phys Rev Lett. 2016 Sep 23;117(13):133003. doi: 10.1103/PhysRevLett.117.133003. Epub 2016 Sep 22.
Coherent optical control of individual particles has been demonstrated both for atoms and semiconductor quantum dots. Here we demonstrate the emergence of quantum coherent effects in semiconductor Rydberg excitons in bulk Cu_{2}O. Because of the spectral proximity between two adjacent Rydberg exciton states, a single-frequency laser may pump both resonances with little dissipation from the detuning. As a consequence, additional resonances appear in the absorption spectrum that correspond to dressed states consisting of two Rydberg exciton levels coupled to the excitonic vacuum, forming a V-type three-level system, but driven only by one laser light source. We show that the level of pure dephasing in this system is extremely low. These observations are a crucial step towards coherently controlled quantum technologies in a bulk semiconductor.
单个粒子的相干光学控制已在原子和半导体量子点中得到证实。在此,我们展示了体相Cu₂O中半导体里德堡激子量子相干效应的出现。由于两个相邻里德堡激子态之间的光谱接近性,单频激光可以泵浦这两个共振,且几乎没有失谐导致的损耗。结果,在吸收光谱中出现了额外的共振,这些共振对应于由两个与激子真空耦合的里德堡激子能级组成的缀饰态,形成了一个V型三能级系统,但仅由一个激光光源驱动。我们表明,该系统中的纯退相水平极低。这些观察结果是迈向体相半导体中相干控制量子技术的关键一步。