Institut für Theoretische Physik II: Weiche Materie, Heinrich-Heine-Universität Düsseldorf, D-40225 Düsseldorf, Germany.
Materials Science Division, Argonne National Laboratory, 9700 S Cass Avenue, Argonne, Illinois 60439, USA.
Nat Commun. 2016 Nov 22;7:13519. doi: 10.1038/ncomms13519.
Fission and fusion processes of particle clusters occur in many areas of physics and chemistry from subnuclear to astronomic length scales. Here we study fission and fusion of magnetic microswimmer clusters as governed by their hydrodynamic and dipolar interactions. Rich scenarios are found that depend crucially on whether the swimmer is a pusher or a puller. In particular a linear magnetic chain of pullers is stable while a pusher chain shows a cascade of fission (or disassembly) processes as the self-propulsion velocity is increased. Contrarily, magnetic ring clusters show fission for any type of swimmer. Moreover, we find a plethora of possible fusion (or assembly) scenarios if a single swimmer collides with a ringlike cluster and two rings spontaneously collide. Our predictions are obtained by computer simulations and verifiable in experiments on active colloidal Janus particles and magnetotactic bacteria.
粒子团的裂变和融合过程发生在物理和化学的许多领域,从亚核到天文长度尺度。在这里,我们研究了由其流体动力学和偶极相互作用控制的磁性微泳体团的裂变和融合。发现了丰富的情景,这些情景主要取决于泳者是推动者还是拉动者。特别是,线性磁链拉动器是稳定的,而当自推进速度增加时,推动器链则显示出一系列的裂变(或拆卸)过程。相反,对于任何类型的泳者,磁性环团都会发生裂变。此外,如果单个泳者与环状团碰撞并且两个环自发碰撞,我们会发现大量可能的融合(或组装)情景。我们的预测是通过计算机模拟得到的,并可在活性胶体 Janus 粒子和趋磁细菌的实验中验证。