Zhang Jiecheng, Levenson-Falk Eli M, Ramshaw B J, Bonn D A, Liang Ruixing, Hardy W N, Hartnoll Sean A, Kapitulnik Aharon
Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA 94305.
Department of Physics, Stanford University, Stanford, CA 94305.
Proc Natl Acad Sci U S A. 2017 May 23;114(21):5378-5383. doi: 10.1073/pnas.1703416114. Epub 2017 May 8.
The thermal diffusivity in the [Formula: see text] plane of underdoped YBCO crystals is measured by means of a local optical technique in the temperature range of 25-300 K. The phase delay between a point heat source and a set of detection points around it allows for high-resolution measurement of the thermal diffusivity and its in-plane anisotropy. Although the magnitude of the diffusivity may suggest that it originates from phonons, its anisotropy is comparable with reported values of the electrical resistivity anisotropy. Furthermore, the anisotropy drops sharply below the charge order transition, again similar to the electrical resistivity anisotropy. Both of these observations suggest that the thermal diffusivity has pronounced electronic as well as phononic character. At the same time, the small electrical and thermal conductivities at high temperatures imply that neither well-defined electron nor phonon quasiparticles are present in this material. We interpret our results through a strongly interacting incoherent electron-phonon "soup" picture characterized by a diffusion constant [Formula: see text], where [Formula: see text] is the soup velocity, and scattering of both electrons and phonons saturates a quantum thermal relaxation time [Formula: see text].
通过局部光学技术在25至300 K的温度范围内测量了欠掺杂YBCO晶体在[公式:见原文]平面内的热扩散率。点热源与其周围一组检测点之间的相位延迟使得能够对热扩散率及其面内各向异性进行高分辨率测量。尽管扩散率的大小可能表明它起源于声子,但其各向异性与报道的电阻率各向异性值相当。此外,在电荷序转变以下,各向异性急剧下降,这再次与电阻率各向异性相似。这两个观察结果都表明热扩散率具有明显的电子和声子特性。同时,高温下较小的电导率和热导率意味着这种材料中既不存在定义明确的电子准粒子,也不存在声子准粒子。我们通过一个由扩散常数[公式:见原文]表征的强相互作用非相干电子 - 声子“汤”模型来解释我们的结果,其中[公式:见原文]是“汤”的速度,并且电子和声子的散射使量子热弛豫时间[公式:见原文]达到饱和。