Jia Xun, Zhang Shuyuan, Sankar Raman, Chou Fang-Cheng, Wang Weihua, Kempa K, Plummer E W, Zhang Jiandi, Zhu Xuetao, Guo Jiandong
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China.
Phys Rev Lett. 2017 Sep 29;119(13):136805. doi: 10.1103/PhysRevLett.119.136805. Epub 2017 Sep 28.
Plasmons, the collective excitations of electrons in the bulk or at the surface, play an important role in the properties of materials, and have generated the field of "plasmonics." We report the observation of a highly unusual acoustic plasmon mode on the surface of a three-dimensional topological insulator (TI) Bi_{2}Se_{3}, using momentum resolved inelastic electron scattering. In sharp contrast to ordinary plasmon modes, this mode exhibits almost linear dispersion into the second Brillouin zone and remains prominent with remarkably weak damping not seen in any other systems. This behavior must be associated with the inherent robustness of the electrons in the TI surface state, so that not only the surface Dirac states but also their collective excitations are topologically protected. On the other hand, this mode has much smaller energy dispersion than expected from a continuous media excitation picture, which can be attributed to the strong coupling with surface phonons.
等离激元,即体材料或表面电子的集体激发,在材料特性中发挥着重要作用,并催生了“等离激元学”领域。我们利用动量分辨非弹性电子散射,报告了在三维拓扑绝缘体(TI)Bi₂Se₃表面观测到一种高度异常的声学等离激元模式。与普通等离激元模式形成鲜明对比的是,这种模式在进入第二布里渊区时呈现出几乎线性的色散,并且在显著弱阻尼下仍很突出,这在其他任何系统中都未见过。这种行为必定与TI表面态中电子固有的稳健性相关联,以至于不仅表面狄拉克态,而且它们的集体激发都受到拓扑保护。另一方面,这种模式的能量色散比连续介质激发图像预期的要小得多,这可归因于与表面声子的强耦合。