In Situ Generation of Plasmonic Nanoparticles for Manipulating Photon-Plasmon Coupling in Microtube Cavities.

In situ generation of silver nanoparticles for selective coupling between localized plasmonic resonances and whispering-gallery modes (WGMs) is investigated by spatially resolved laser dewetting on microtube cavities. The size and morphology of the silver nanoparticles are changed by adjusting the laser power and irradiation time, which in turn effectively tune the photon-plasmon coupling strength. Depending on the relative position of the plasmonic nanoparticles spot and resonant field distribution of WGMs, selective coupling between the localized surface plasmon resonances (LSPRs) and WGMs is experimentally demonstrated. Moreover, by creating multiple plasmonic-nanoparticle spots on the microtube cavity, the field distribution of optical axial modes is freely tuned due to multicoupling between LSPRs and WGMs. The multicoupling mechanism is theoretically investigated by a modified quasipotential model based on perturbation theory. This work provides an in situ fabrication of plasmonic nanoparticles on three-dimensional microtube cavities for manipulating photon-plasmon coupling which is of interest for optical tuning abilities and enhanced light-matter interactions.