State Key Laboratory of Earth Surface Processes and Resource Ecology, Beijing Normal University, Beijing 100875, China; Faculty of Geographical Science, Beijing Normal University, Beijing 100875, China.
Key Laboratory of Environmental Change and Natural Disaster, Ministry of Education, Beijing Normal University, Beijing 100875, China.
Chemosphere. 2018 Aug;205:52-61. doi: 10.1016/j.chemosphere.2018.04.071. Epub 2018 Apr 14.
This study explored the interdecadal variations and their horizontal and vertical light extinction performances of atmospheric particulate matter with aerodynamic diameters ≤2.5 μm (PM), particulate matter with aerodynamic diameters ≤ 10 μm (PM), and total suspended particulates (TSPs) in Beijing from 1980 to 2015, using data available from historical publications. Prominent declines of PM, PM, and TSPs were detected with long-term linear trends of -6.7, -4.3, and -1.9 μg m yr, respectively. Generally, on the annual scale during the studied period, it was found that PM displayed negative correlation (R = 0.38, p < 0.01) with visibility and positive correlation (R = 0.41, p < 0.01) with aerosol optical depth (AOD). Comparably, PM exhibited robust negative correlation (R = 0.61, p < 0.01) with visibility and positive correlation (R = 0.82, p < 0.01) with AOD. The complicated interdecadal variations and light extinction performances of PM were found, suggesting the changes on particle composition and vertical distribution of PM in the atmosphere.
本研究利用历史出版物中的数据,探讨了 1980 年至 2015 年北京大气中空气动力学直径≤2.5μm(PM)、空气动力学直径≤10μm(PM)和总悬浮颗粒物(TSPs)的年代际变化及其水平和垂直消光性能。PM、PM和 TSPs 均呈显著下降趋势,长期线性趋势分别为-6.7μg/m·yr、-4.3μg/m·yr 和-1.9μg/m·yr。总的来说,在研究期间的年际尺度上,发现 PM 与能见度呈负相关(R=0.38,p<0.01),与气溶胶光学深度(AOD)呈正相关(R=0.41,p<0.01)。相比之下,PM 与能见度呈显著负相关(R=0.61,p<0.01),与 AOD 呈正相关(R=0.82,p<0.01)。发现 PM 的复杂年代际变化及其消光性能表明,大气中 PM 的颗粒组成和垂直分布发生了变化。