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分析亚热带西太平洋地区远距离传输的生物质燃烧和灰尘的共存情况。

Analysis of the Co-existence of Long-range Transport Biomass Burning and Dust in the Subtropical West Pacific Region.

机构信息

Department of Civil and Environmental Engineering, the University of Tennessee, Knoxville, TN, 37996, USA.

Climate Change Science Institute, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA.

出版信息

Sci Rep. 2018 Jun 12;8(1):8962. doi: 10.1038/s41598-018-27129-2.

Abstract

Biomass burning and wind-blown dust has been well investigated during the past decade regarding their impacts on environment, but their co-existence hasn't been recognized because they usually occur in different locations and episodes. In this study we reveal the unique co-existence condition that dust from the Taklamakan and Gobi Desert (TGD) and biomass burning from Peninsular Southeast Asia (PSEA) can reach to the west Pacific region simultaneously in boreal spring (March and April). The upper level trough at 700hPa along east coast of China favors the large scale subsidence of TGD dust while it travels southeastwards, and drives the PSEA biomass burning plume carried by the westerlies at 3-5 km to descend rapidly to around 1.5 km and mix with dust around southeast China and Taiwan. As compared to the monthly averages in March and April, surface observations suggested that concentrations of PM, PM, O, and CO were 69%, 37%, 20%, and 18% higher respectively during the 10 identified co-existence events which usually lasted for 2-3 days. Co-existence also lowers the surface O, NOx, and SO by 4-5% due to the heterogeneous chemistry between biomass burning and mineral dust as indicated by model simulations.

摘要

在过去的十年中,生物质燃烧和风沙已被充分研究,其对环境的影响也得到了广泛关注,但由于它们通常发生在不同的地点和时段,因此它们的共存问题尚未得到认识。在本研究中,我们揭示了一种独特的共存情况,即在春季(三月和四月),来自塔克拉玛干和戈壁沙漠(TGD)的尘埃和来自东南亚半岛(PSEA)的生物质燃烧可以同时到达西太平洋地区。在中国东海岸 700hPa 的高空槽有利于 TGD 尘埃在向东南方向传输时的大规模下沉,同时也将西风带来的 PSEA 生物质燃烧羽流驱动至 3-5km 高度迅速下降至约 1.5km 高度,并与中国东南部和台湾地区的尘埃混合。与三月和四月的月平均值相比,地面观测表明,在 10 次被识别的共存事件中,PM、PM、O 和 CO 的浓度分别高出 69%、37%、20%和 18%,这些事件通常持续 2-3 天。共存还通过模型模拟表明,由于生物质燃烧和矿物质尘埃之间的非均相化学作用,降低了地表 O、NOx 和 SO 的浓度,降幅分别为 4-5%。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/227c/5997683/75b061a09685/41598_2018_27129_Fig1_HTML.jpg

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