Cramer Tobias, Fratelli Ilaria, Barquinha Pedro, Santa Ana, Fernandes Cristina, D'Annunzio Franck, Loussert Christophe, Martins Rodrigo, Fortunato Elvira, Fraboni Beatrice
Department of Physics and Astronomy, University of Bologna, Viale Berti Pichat 6/2, 40127 Bologna, Italy.
CENIMAT/I3N and CEMOP-UNINOVA, Departamento de Ciência dos Materiais, Faculdade de Ciências e Tecnologia, Universidade Nova de Lisboa, Campus de Caparica, 2829-516 Caparica, Portugal.
Sci Adv. 2018 Jun 29;4(6):eaat1825. doi: 10.1126/sciadv.aat1825. eCollection 2018 Jun.
Distributed x-ray radiation dosimetry is crucial in diverse security areas with significant environmental and human impacts such as nuclear waste management, radiotherapy, or radioprotection devices. We present a fast, real-time dosimetry detection system based on flexible oxide thin-film transistors that show a quantitative shift in threshold voltage of up to 3.4 V/gray upon exposure to ionizing radiation. The transistors use indium-gallium-zinc-oxide as a semiconductor and a multilayer dielectric based on silicon oxide and tantalum oxide. Our measurements demonstrate that the threshold voltage shift is caused by the accumulation of positive ionization charge in the dielectric layer due to high-energy photon absorption in the high- dielectric. The high mobility combined with a steep subthreshold slope of the transistor allows for fast, reliable, and ultralow-power readout of the deposited radiation dose. The order-of-magnitude variation in transistor channel impedance upon exposure to radiation makes it possible to use a low-cost, passive radiofrequency identification sensor tag for its readout. In this way, we demonstrate a passive, programmable, wireless sensor that reports in real time the excess of critical radiation doses.
分布式X射线辐射剂量测定在核废料管理、放射治疗或辐射防护设备等对环境和人类有重大影响的各种安全领域至关重要。我们展示了一种基于柔性氧化物薄膜晶体管的快速实时剂量测定检测系统,该晶体管在暴露于电离辐射时阈值电压会出现高达3.4伏/格雷的定量偏移。这些晶体管使用铟镓锌氧化物作为半导体,并采用基于氧化硅和氧化钽的多层电介质。我们的测量表明,阈值电压偏移是由于高介电常数材料中高能光子吸收导致电介质层中积累正电离电荷所致。晶体管的高迁移率与陡峭的亚阈值斜率相结合,使得能够快速、可靠且超低功耗地读出沉积的辐射剂量。暴露于辐射时晶体管沟道阻抗的数量级变化使得可以使用低成本的无源射频识别传感器标签进行读出。通过这种方式,我们展示了一种无源、可编程的无线传感器,可实时报告超过临界辐射剂量的情况。