Department of Chemistry, Tsinghua University, Beijing, 100084, China.
INPAC-Institute for Nanoscale Physics and Chemistry, K.U. Leuven, Celestijnenlaan 200 D, B-3001, Leuven, Belgium.
Adv Mater. 2019 Feb;31(7):e1806341. doi: 10.1002/adma.201806341. Epub 2018 Dec 27.
Manipulation of light below the diffraction limit forms the basis of nanophotonics. Metals can confine light at the subwavelength scale but suffer from high loss of energy. Recent reports have theoretically demonstrated the possibility of light confinement below the diffraction limit using transparent dielectric metamaterials. Here, nanoscale light confinement (<λ/20) in transparent dielectric materials is shown experimentally through a luminescent nanosystem with rationally designed dielectric claddings. Theoretically, green light with a wavelength of 540 nm has a transmission of 98.8% when passing through an ultrathin NaYF /NaGdF superlattice cladding (thickness: 6.9 nm). Unexpectedly, the complete confinement of green emission (540 nm) by such an ultrathin dielectric cladding is directly observed. FDTD calculations are used to confirm that the ultrathin dielectric cladding has negligible influence on the transmission of propagating light, but extraordinary confinement of evanescent waves. This will provide new opportunities for nanophotonics by completely averting the use of metals.
低于衍射极限的光操控是纳米光子学的基础。金属可以在亚波长尺度下限制光,但会遭受能量的高损耗。最近的报告从理论上证明了使用透明介电超材料实现低于衍射极限的光限制的可能性。在这里,通过具有合理设计的介电包层的发光纳米系统,实验上实现了透明介电材料中的纳米级光限制(<λ/20)。理论上,当 540nm 波长的绿光通过超薄 NaYF/NaGdF 超晶格包层(厚度:6.9nm)时,其透过率为 98.8%。出人意料的是,这种超薄介电包层直接观察到了绿光发射(540nm)的完全限制。FDTD 计算用于确认超薄介电包层对传播光的传输几乎没有影响,但对消逝波有非凡的限制。这将通过完全避免使用金属,为纳米光子学提供新的机会。