Autonomous multi-species environmental gas sensing using drone-based Fourier-transform infrared spectroscopy.

Unmanned aerial vehicles (UAVs)-or drones-present compelling new opportunities for airborne gas sensing in applications such as environmental monitoring, hazardous scene assessment, and facilities' inspection. Instrumenting a UAV for this purpose encounters trade-offs between sensor size, weight, power, and performance, which drives the adoption of lightweight electrochemical and photo-ionisation detectors. However, this occurs at the expense of speed, selectivity, sensitivity, accuracy, resolution, and traceability. Here, we report on the design and integration of a broadband Fourier-transform infrared spectrometer with an autonomous UAV, providing ro-vibrational spectroscopy throughout the molecular fingerprint region from 3 - 11 µm (3333 - 909 cm) and enabling rapid, quantitative aerial surveys of multiple species simultaneously with an estimated noise-limited performance of 18 ppm (propane). Bayesian interpolation of the acquired gas concentrations is shown to provide both localization of a point source with approximately one meter accuracy, and distribution mapping of a gas cloud, with accompanying uncertainty quantification.