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基于聚甲基丙烯酸甲酯:CdSe/CdZnS 量子点纳米复合材料的柔性有机突触器件。

Flexible organic synaptic device based on poly (methyl methacrylate):CdSe/CdZnS quantum-dot nanocomposites.

机构信息

Department of Electronics and Computer Engineering, Hanyang University, Seoul, 04763, Korea.

College of Physics and Information Engineering, Fuzhou University, Fuzhou, 350108, China.

出版信息

Sci Rep. 2019 Jul 5;9(1):9755. doi: 10.1038/s41598-019-46226-4.

Abstract

A synaptic device that functionally mimics a biological synapse is a promising candidate for use as an electronic element in a neuromorphic system. In this study, flexible electronic synaptic devices based on poly (methyl methacrylate) (PMMA):CdSe/CdZnS core-shell quantum-dot (QD) nanocomposites are demonstrated. The current-voltage characteristics for the synaptic devices under consecutive voltage sweeps show clockwise hysteresis, which is a critical feature of an artificial synaptic device. The effect of the CdSe/CdZnS QD concentration on the device performance is studied. The flexible electronic synaptic devices under bending show the similar and stable electrical performances. The memory retention measurements show that the e-synapse exhibits long-term potentiation and depression. The carrier transport mechanisms are analyzed, and thermionic emission and space-charge-limited-current conduction are found to be dominant.

摘要

一种在功能上模仿生物突触的突触器件,是作为神经形态系统中电子元件使用的有前途的候选者。在这项研究中,展示了基于聚甲基丙烯酸甲酯(PMMA):CdSe/CdZnS 核壳量子点(QD)纳米复合材料的柔性电子突触器件。在连续电压扫描下,突触器件的电流-电压特性表现出顺时针滞后,这是人工突触器件的关键特性。研究了 CdSe/CdZnS QD 浓度对器件性能的影响。在弯曲状态下,柔性电子突触器件表现出相似且稳定的电性能。记忆保持测量表明,电子突触表现出长时程增强和长时程抑制。分析了载流子输运机制,发现热电子发射和空间电荷限制电流传导占主导地位。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6a2f/6611803/207d2ea74907/41598_2019_46226_Fig1_HTML.jpg

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