Zhang Bo, Chen Ke, Chen Yewei, Yang Beilei, Guo Min, Deng Hong, Ma Fengxiang, Zhu Feng, Gong Zhenfeng, Peng Wei, Yu Qingxu
Opt Express. 2020 Mar 2;28(5):6618-6630. doi: 10.1364/OE.382310.
A high-sensitivity photoacoustic (PA) spectroscopy (PAS) system is proposed for dual enhancement from both PA signal excitation and detection by employing a miniaturized Herriott cell and a fiber-optic microphone (FOM). The length of the optical absorption path of the PA cell is optimized to ∼374 mm with 17 reflections. The volume of the PA cell is only 622 µL. The FOM is a low-finesse fiber-optic Fabry-Pérot (FP) interferometer. The two reflectors of the FP cavity are formed by a fiber endface and a circular titanium diaphragm with a radius of 4.5 mm and a thickness of 3 µm. A fast demodulated white-light interferometer (WLI) is utilized to measure the absolute FP cavity length. The acoustic responsivity of the FOM reaches 126.6 nm/Pa. Several representative PA signals of trace acetylene (CH) are detected to evaluate the performance of the trace gas detector in the near-infrared region. Experimental results show that the minimum detectable pressure (MDP) of the FOM is 3.8 µPa/Hz at 110 Hz. The noise equivalent minimum detection concentration is measured to be 8.4 ppb with an integration time of 100 s. The normalized noise equivalent absorption (NNEA) coefficient is calculated as 1.4×10 cm·W·Hz.
提出了一种高灵敏度光声(PA)光谱(PAS)系统,通过采用小型化赫里奥特池和光纤麦克风(FOM),实现光声信号激发和检测的双重增强。光声池的光吸收路径长度经优化至约374 mm,有17次反射。光声池的体积仅为622 µL。该光纤麦克风是一种低精细度光纤法布里 - 珀罗(FP)干涉仪。FP腔的两个反射镜由一个光纤端面和一个半径为4.5 mm、厚度为3 µm的圆形钛膜构成。利用快速解调白光干涉仪(WLI)测量绝对FP腔长度。该光纤麦克风的声响应率达到126.6 nm/Pa。检测了几种代表性的痕量乙炔(CH)光声信号,以评估近红外区域痕量气体探测器的性能。实验结果表明,在110 Hz时,该光纤麦克风的最小可检测压力(MDP)为3.8 µPa/Hz。在积分时间为100 s时,测得噪声等效最小检测浓度为8.4 ppb。归一化噪声等效吸收(NNEA)系数计算为1.4×10 cm·W·Hz。