Baker K R, Nguyen T K V, Sareen N, Henderson B H
U.S. Environmental Protection Agency, Research Triangle Park, NC, USA.
U.S. Environmental Protection Agency, San Francisco, CA, USA.
Atmos Environ (1994). 2020 Aug 1;234:117543-11753. doi: 10.1016/j.atmosenv.2020.117543.
A photochemical model platform for Hawaii, Puerto Rico, and Virgin Islands predicting O, PM, and regional haze would be useful to support assessments relevant for the National Ambient Air Quality Standards (NAAQS), Regional Haze Rule, and the Prevention of Significant Deterioration (PSD) program. These areas have not traditionally been modeled with photochemical transport models, but a reasonable representation of meteorology, emissions (natural and anthropogenic), chemistry, and deposition could support air quality management decisions in these areas. Here, a prognostic meteorological model (Weather Research and Forecasting) and photochemical transport (Community Multiscale Air Quality) model were applied for the entire year of 2016 at 27, 9, and 3 km grid resolution for areas covering the Hawaiian Islands and Puerto Rico/Virgin Islands. Model predictions were compared against surface and upper air meteorological and chemical measurements available in both areas. The vertical gradient of temperature, humidity, and winds in the troposphere was well represented. Surface layer meteorological model performance was spatially variable, but temperature tended to be underestimated in Hawaii. Chemically speciated daily average PM was generally well characterized by the modeling system at urban and rural monitors in Hawaii and Puerto Rico/Virgin Islands. Model performance was notably impacted by the wildfire emission methodology. Model performance was mixed for hourly SO, NO, PM, and CO and was often related to how well local emissions sources were characterized. SO predictions were much lower than measurements at monitors near active volcanos on Hawaii, which was expected since volcanic emissions were not included in these model simulations. Further research is needed to assess emission inventory representation of these areas and how microscale meteorology influenced by the complex land-water and terrain interfaces impacts higher time resolution performance.
一个用于夏威夷、波多黎各和美属维尔京群岛的光化学模型平台,用于预测臭氧、颗粒物和区域霾,将有助于支持与国家环境空气质量标准(NAAQS)、区域霾规则和防止重大恶化(PSD)计划相关的评估。这些地区传统上未使用光化学传输模型进行模拟,但对气象学、排放(自然和人为)、化学和沉降的合理表征可以支持这些地区的空气质量管理决策。在此,一个预后气象模型(天气研究与预报)和光化学传输模型(社区多尺度空气质量)在2016年全年以27公里、9公里和3公里的网格分辨率应用于覆盖夏威夷群岛以及波多黎各/美属维尔京群岛的区域。将模型预测结果与这两个地区现有的地面和高空气象及化学测量数据进行了比较。对流层中温度、湿度和风的垂直梯度得到了很好的体现。表层气象模型的性能在空间上存在差异,但夏威夷的温度往往被低估。在夏威夷以及波多黎各/美属维尔京群岛的城市和农村监测站,化学形态的日均颗粒物通常能被该建模系统很好地表征。野火排放方法对模型性能有显著影响。对于每小时的二氧化硫、一氧化氮、颗粒物和一氧化碳,模型性能参差不齐,并且往往与当地排放源的表征情况有关。在夏威夷活火山附近的监测站,二氧化硫的预测值远低于测量值,这是预期的,因为这些模型模拟未包括火山排放。需要进一步研究来评估这些地区排放清单的代表性,以及复杂的陆地 - 水体和地形界面所影响的微尺度气象学如何影响更高时间分辨率的性能。