Photocatalysis International Research Center, Tokyo University of Science, Yamazaki, Noda, Chiba 278-8510, Japan.
Department of Automotive Engineering, Yeungnam University, 280 Daehak-ro, Gyeongsan, Gyeonbuk 38541, Republic of Korea.
J Colloid Interface Sci. 2021 Jan 15;582(Pt B):1058-1066. doi: 10.1016/j.jcis.2020.08.102. Epub 2020 Aug 29.
Different types of organic impurities such as dyes, acids, and alcohols are discharged into potable water sources. The removal of these hazardous organic pollutants from wastewater is an important task globally. However, the conventional methods used to remove organic impurities suffer from low efficiency and recycling problems. Photocatalysis is a promising advanced oxidation process for the degradation of organic compounds in aqueous solution. Titanium dioxide (TiO) is commonly used as a photocatalyst. However, the wide bandgap of TiO means that it is activated by ultraviolet light, which restrains its ability to harvest solar energy. In this study, a simple water-based precipitation method was used to synthesize TiO@nanodiamond composites. The ability of the composites to degrade bisphenol A as a model organic pollutant was investigated. It was found that 10 ppm of bisphenol A was completely degraded in 100 min by the TiO@nanodiamond photocatalyst under ultraviolet illumination.
不同类型的有机杂质,如染料、酸和醇,被排放到饮用水源中。从废水中去除这些危险的有机污染物是全球范围内的一项重要任务。然而,用于去除有机杂质的传统方法存在效率低和回收问题。光催化是一种很有前途的高级氧化工艺,可用于降解水溶液中的有机化合物。二氧化钛 (TiO) 通常用作光催化剂。然而,TiO 的宽带隙意味着它只能被紫外光激活,这限制了它利用太阳能的能力。在这项研究中,采用了一种简单的水基沉淀法来合成 TiO@纳米金刚石复合材料。研究了复合材料降解双酚 A 作为模型有机污染物的能力。结果发现,在紫外光照射下,10ppm 的双酚 A 在 100 分钟内被 TiO@纳米金刚石光催化剂完全降解。