Yang Wei, Mo Chong-Jie, Fu Shi-Bin, Yang Yu, Zheng Fa-Wei, Wang Xiao-Hui, Liu Yuan-An, Hao Ning, Zhang Ping
Beijing Key Laboratory of Work Safety Intelligent Monitoring, Beijing University of Posts and Telecommunications, Beijing 100876, China.
Beijing Computational Science Research Center, Beijing 100193, China.
Phys Rev Lett. 2020 Dec 4;125(23):237006. doi: 10.1103/PhysRevLett.125.237006.
Recent experiments have tuned the monolayer 1T^{'}-WTe_{2} to be superconducting by electrostatic gating. Here, we theoretically study the phonon-mediated superconductivity in monolayer 1T^{'}-WTe_{2} via charge doping. We reveal that the emergence of soft-mode phonons with specific momentum is crucial to give rise to the superconductivity in the electron-doping regime, whereas no such soft-mode phonons and no superconductivity emerge in the hole-doping regime. We also find a superconducting dome, which can be attributed to the change of Fermi surface nesting conditions with electron doping. By taking into account the experimentally established strong anisotropy of temperature-dependent upper critical field H_{c2} between the in-plane and out-of-plane directions, we show that the superconducting state probably has the unconventional equal-spin-triplet pairing in the A_{u} channel of the C_{2h} point group. Our studies provide a promising understanding to the doping dependent superconductivity and strong anisotropy of H_{c2} in monolayer 1T^{'}-WTe_{2}, and can be extended to understand the superconductivity in other gated transition metal dichalcogenides.
最近的实验通过静电门控将单层1T'-WTe₂调节至超导状态。在此,我们从理论上研究了通过电荷掺杂在单层1T'-WTe₂中由声子介导的超导性。我们发现,具有特定动量的软模声子的出现对于在电子掺杂体系中产生超导性至关重要,而在空穴掺杂体系中则不会出现此类软模声子,也不会出现超导性。我们还发现了一个超导穹顶,这可归因于费米面嵌套条件随电子掺杂的变化。考虑到实验确定的面内和面外方向上与温度相关的上临界场Hc₂的强各向异性,我们表明超导态可能在C₂h点群的Au通道中具有非常规的等自旋三重态配对。我们的研究为单层1T'-WTe₂中与掺杂相关的超导性和Hc₂的强各向异性提供了有前景的理解,并且可以扩展到理解其他门控过渡金属二卤化物中的超导性。