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室温有机晶格拓扑极化激元激光。

Room-Temperature Topological Polariton Laser in an Organic Lattice.

机构信息

Institute of Physics, University of Oldenburg, D-26129 Oldenburg, Germany.

SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY 16 9SS, United Kingdom.

出版信息

Nano Lett. 2021 Aug 11;21(15):6398-6405. doi: 10.1021/acs.nanolett.1c00661. Epub 2021 Jul 30.

Abstract

Interacting bosonic particles in artificial lattices have proven to be a powerful tool for the investigation of exotic phases of matter as well as phenomena resulting from nontrivial topology. Exciton-polaritons, bosonic quasi-particles of light and matter, have been shown to combine the on-chip benefits of optical systems with strong interactions, inherited from their matter character. Technologically significant semiconductor platforms strictly require cryogenic temperatures. In this communication, we demonstrate exciton-polariton lasing for topological defects emerging from the imprinted lattice structure at room temperature. We utilize red fluorescent protein derived from DsRed of Discosoma sea anemones, hosting highly stable Frenkel excitons. Using a patterned mirror cavity, we tune the lattice potential landscape of a linear Su-Schrieffer-Heeger chain to design topological defects at domain boundaries and at the edge. We unequivocally demonstrate polariton lasing from these topological defects. This progress has paved the road to interacting boson many-body physics under ambient conditions.

摘要

在人工晶格中相互作用的玻色子已被证明是研究物质奇异相以及源自非平凡拓扑的现象的有力工具。激子极化激元,光和物质的玻色准粒子,已被证明将光学系统的片上优势与继承自物质特性的强相互作用结合在一起。具有技术意义的半导体平台严格要求低温。在本通讯中,我们展示了室温下从压印晶格结构中出现的拓扑缺陷的激子极化激元激射。我们利用源自 Discosoma 海葵的 DsRed 的红色荧光蛋白,其具有高度稳定的 Frenkel 激子。使用图案化的反射镜腔,我们调谐线性 Su-Schrieffer-Heeger 链的晶格势景观,以在域边界和边缘设计拓扑缺陷。我们明确地证明了来自这些拓扑缺陷的极化激元激射。这一进展为在环境条件下进行相互作用的玻色子多体物理铺平了道路。

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