Department of Anesthesiology, University of Michigan and VAMC, 2215 Fuller Road, Ann Arbor, MI 48105, USA.
Department of Anesthesiology, Perioperative and Pain Medicine, Stanford University School of Medicine, 300 Pasteur Drive, Stanford, CA 94305, USA.
Int J Mol Sci. 2021 Sep 30;22(19):10625. doi: 10.3390/ijms221910625.
Cytochrome P450 reductase (CYPOR) provides electrons to all human microsomal cytochrome P450s (cyt P450s). The length and sequence of the "140s" FMN binding loop of CYPOR has been shown to be a key determinant of its redox potential and activity with cyt P450s. Shortening the "140s loop" by deleting glycine-141(ΔGly141) and by engineering a second mutant that mimics flavo-cytochrome P450 BM3 (ΔGly141/Glu142Asn) resulted in mutants that formed an unstable anionic semiquinone. In an attempt to understand the molecular basis of the inability of these mutants to support activity with cyt P450, we expressed, purified, and determined their ability to reduce ferric P450. Our results showed that the ΔGly141 mutant with a very mobile loop only reduced ~7% of cyt P450 with a rate similar to that of the wild type. On the other hand, the more stable loop in the ΔGly141/Glu142Asn mutant allowed for ~55% of the cyt P450 to be reduced ~60% faster than the wild type. Our results reveal that the poor activity of the ΔGly141 mutant is primarily accounted for by its markedly diminished ability to reduce ferric cyt P450. In contrast, the poor activity of the ΔGly141/Glu142Asn mutant is presumably a consequence of the altered structure and mobility of the "140s loop".
细胞色素 P450 还原酶 (CYPOR) 为所有人类微粒体细胞色素 P450(细胞色素 P450)提供电子。已经表明,CYPOR 的“140s”FMN 结合环的长度和序列是其还原电势和与细胞色素 P450 相互作用的关键决定因素。通过删除甘氨酸-141(ΔGly141)和工程设计模拟黄素-细胞色素 P450 BM3(ΔGly141/Glu142Asn)的第二个突变体来缩短“140s 环”,导致形成不稳定的阴离子半醌的突变体。为了试图了解这些突变体无法支持细胞色素 P450 活性的分子基础,我们表达、纯化并确定了它们还原高铁细胞色素 P450 的能力。我们的结果表明,具有非常可移动环的 ΔGly141 突变体仅还原了约 7%的细胞色素 P450,其还原速率与野生型相似。另一方面,在 ΔGly141/Glu142Asn 突变体中更稳定的环允许约 55%的细胞色素 P450被还原,其速度比野生型快约 60%。我们的结果表明,ΔGly141 突变体活性差的主要原因是其还原高铁细胞色素 P450 的能力明显降低。相比之下,ΔGly141/Glu142Asn 突变体的活性差可能是由于“140s 环”的结构和流动性改变所致。