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基于中国实际测量的非道路施工设备不可忽视的黑碳排放。

Non-negligible emissions of black carbon from non-road construction equipment based on real-world measurements in China.

作者信息

Wu Bobo, Xuan Kaijie, Shen Xianbao, Zhao Qiangqiang, Shi Yue, Kong Lei, Hu Jinfeng, Li Xin, Zhang Hanyu, Cao Xinyue, Hao Xuewei, Zhou Qi, Yao Zhiliang

机构信息

School of Ecology and Environment, Beijing Technology and Business University, Beijing 100048, China; State Environmental Protection Key Laboratory of Food Chain Pollution Control, Beijing Technology and Business University, Beijing 100048, China; Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry, Beijing Technology and Business University, Beijing 100048, China.

School of Ecology and Environment, Beijing Technology and Business University, Beijing 100048, China.

出版信息

Sci Total Environ. 2022 Feb 1;806(Pt 3):151300. doi: 10.1016/j.scitotenv.2021.151300. Epub 2021 Oct 28.

Abstract

Non-road construction equipment (NRCE) has become a vital contributor to urban air pollutants with the rapid urbanization in China. Black carbon (BC), as a key pollutant emitted from NRCE (mainly diesel-fueled), has attracted considerable concerns due to adverse impacts on climate change, visibility, and human health. However, the understanding of its emissions is still unclear based on limited research results. In this study, we conducted real-world measurements on BC emissions from 12 excavators and 9 loaders to characterize the variation and quantify fuel-based emission factors (EFs) by using a synchronous platform based on PEMS (SP-PEMS). We analyzed the impacts of key factors (operation mode, emission standard, and engine rated power) on BC emission comprehensively. High BC emission in working mode may be mainly owing to the increase of fuel consumption and the deterioration of air-fuel ratio. With more stringent emission standards, BC EFs of all tested NRCE present significant decreasing trends. Interestingly, NRCE with high rated power generally exhibits lower BC emissions. Through comparison, we find BC EFs in this study are generally higher than elemental carbon (EC) EFs reported in previous studies, which will lead BC emissions from NRCE to be underestimated while EC EFs are used instead of BC EFs. Furthermore, BC EFs of NRCE with Stage III are significantly higher (1-3 orders of magnitude) than those of on-road diesel trucks with the current mainstream emission standards of China IV and China V, which reinforces the urgency and importance of controlling BC emissions from NRCE in China. Finally, we recommend BC EFs of excavators and loaders under different emission standards and operation modes, and which preliminarily fills the gap in localized BC EFs of typical NRCE to relieve the urgent needs for emission inventory calculation.

摘要

随着中国城市化进程的快速推进,非道路施工设备(NRCE)已成为城市空气污染物的重要来源。黑碳(BC)作为NRCE(主要以柴油为燃料)排放的一种关键污染物,因其对气候变化、能见度和人类健康的不利影响而备受关注。然而,基于有限的研究结果,对其排放情况仍不清楚。在本研究中,我们使用基于车载排放测量系统的同步平台(SP-PEMS),对12台挖掘机和9台装载机的黑碳排放进行了实际测量,以表征其变化特征并量化基于燃料的排放因子(EFs)。我们全面分析了关键因素(运行模式、排放标准和发动机额定功率)对黑碳排放的影响。工作模式下的高黑碳排放可能主要归因于燃料消耗的增加和空燃比的恶化。随着排放标准的日益严格,所有测试的NRCE的黑碳排放因子均呈现出显著下降的趋势。有趣的是,额定功率高的NRCE通常黑碳排放量较低。通过比较,我们发现本研究中的黑碳排放因子普遍高于先前研究中报道的元素碳(EC)排放因子,这将导致在使用EC排放因子而非BC排放因子时,NRCE的黑碳排放被低估。此外,符合国三标准的NRCE的黑碳排放因子比符合中国现行主流排放标准国四和国五的道路柴油卡车的黑碳排放因子显著更高(1至3个数量级),这凸显了在中国控制NRCE黑碳排放的紧迫性和重要性。最后,我们给出了不同排放标准和运行模式下挖掘机和装载机的黑碳排放因子推荐值,初步填补了典型NRCE本地化黑碳排放因子的空白,以满足排放清单计算的迫切需求。

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