揭示新兴二维有机-无机卤化物钙钛矿在能源应用方面的情况。
Shedding light on the energy applications of emerging 2D hybrid organic-inorganic halide perovskites.
作者信息
Li Neng, Yang Yufei, Shi Zuhao, Lan Zhigao, Arramel Arramel, Zhang Peng, Ong Wee-Jun, Jiang Jizhou, Lu Jianfeng
机构信息
State Key Laboratory of Silicate Materials for Architecture, Wuhan University of Technology, Wuhan 430070, China.
Shenzhen Research Institute of Wuhan University of Technology, Shenzhen 518000, China.
出版信息
iScience. 2022 Jan 7;25(2):103753. doi: 10.1016/j.isci.2022.103753. eCollection 2022 Feb 18.
Unique performance of the hybrid organic-inorganic halide perovskites (HOIPs) has attracted great attention because of their continuous exploration and breakthrough in a multitude of energy-related applications. However, the instability and lead-induced toxicity that arise in bulk perovskites are the two major challenges that impede their future commercialization process. To find a solution, a series of two-dimensional HOIPs (2D HOIPs) are investigated to prolong the device lifetime with highly efficient photoelectric conversion and energy storage. Herein, the recent advances of 2D HOIPs and their structural derivatives for the energy realms are summarized and discussed. The basic understanding of crystal structures, physicochemical properties, and growth mechanisms is presented. In addition, the current challenges and future directions to provide a roadmap for the development of next generation 2D HOIPs are prospected.
有机-无机卤化物杂化钙钛矿（HOIPs）的独特性能因其在众多能源相关应用中的不断探索和突破而备受关注。然而，体相钙钛矿中出现的不稳定性和铅诱导的毒性是阻碍其未来商业化进程的两大主要挑战。为了找到解决方案，人们研究了一系列二维HOIPs（2D HOIPs），以通过高效的光电转换和能量存储来延长器件寿命。在此，总结并讨论了二维HOIPs及其结构衍生物在能源领域的最新进展。介绍了对晶体结构、物理化学性质和生长机制的基本理解。此外，展望了当前的挑战和未来方向，为下一代二维HOIPs的发展提供路线图。
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